Ultrafast Thermal Switching Enabled by Transient Polaritons
Ultrafast thermal switches are pivotal for managing heat generated in advanced solid-state applications, including high-speed chiplets, thermo-optical modulators, and on-chip lasers. However, conventional phonon-based switches cannot meet the demand for picosecond-level response times, and existing near-field radiative thermal switches face challenges in efficiently modulating heat transfer across vacuum gaps. To overcome these limitations, we propose an ultrafast thermal switch design based on pump-driven transient polaritons in asymmetric terminals. Demonstrated with WSe<sub>2</sub> and graphene, this approach achieves an impressive thermal switching ratio exceeding 10,000 with response times on the picosecond scale, outperforming current designs by at least 2 orders of magnitude. This exceptional performance is driven by dynamic polaritonic coupling between terminals, activated by ultrafast photoexcitation. Additionally, the WSe<sub>2</sub> monolayer-based switch exhibits a laser cooling effect, enabled by enhanced carrier excitation efficiency and prolonged carrier lifetimes, introducing a disruptive mechanism for laser cooling. Our findings highlight the strong potential of photodriven transient polaritons in advancing ultrafast thermal switches and nanoscale cooling technologies.
Authors
- Bei Yang (ORCID: https://orcid.org/0000-0002-0976-0650)
- Bai Song (ORCID: https://orcid.org/0000-0003-3013-9831)
- F. Javier Garcı́a de Abajo (ORCID: https://orcid.org/0000-0002-4970-4565)
- Qing Dai (ORCID: https://orcid.org/0000-0002-1750-0867)
Institutions
- Institució Catalana de Recerca i Estudis Avançats (ES)
- Institute of Photonic Sciences (ES)
- Shanghai Jiao Tong University (CN)
- Peking University (CN)
- Center for NanoScience (DE)
- Shanghai Institute for Science of Science (CN)
- Beijing Microelectronics Technology Institute (CN)
- Physical Measurement Laboratory (US)
- Barcelona Institute of Science and Technology (ES)
- National Center for Nanoscience and Technology (CN)
- University of Chinese Academy of Sciences (CN)
- Institute of Science and Technology
Publication Details
- Journal
- ACS Nano
- Published
- 2024-12-27
- DOI
- https://doi.org/10.1021/acsnano.4c14188
- Citations
- 4
- Primary Topic
- Thermal Radiation and Cooling Technologies
- Type
- article
- Field-Weighted Citation Impact
- 1.04
Funders
- National Natural Science Foundation of China
- Chinese Academy of Sciences
- National Key Research and Development Program of China