Ultrafast Thermal Switching Enabled by Transient Polaritons

Ultrafast thermal switches are pivotal for managing heat generated in advanced solid-state applications, including high-speed chiplets, thermo-optical modulators, and on-chip lasers. However, conventional phonon-based switches cannot meet the demand for picosecond-level response times, and existing near-field radiative thermal switches face challenges in efficiently modulating heat transfer across vacuum gaps. To overcome these limitations, we propose an ultrafast thermal switch design based on pump-driven transient polaritons in asymmetric terminals. Demonstrated with WSe<sub>2</sub> and graphene, this approach achieves an impressive thermal switching ratio exceeding 10,000 with response times on the picosecond scale, outperforming current designs by at least 2 orders of magnitude. This exceptional performance is driven by dynamic polaritonic coupling between terminals, activated by ultrafast photoexcitation. Additionally, the WSe<sub>2</sub> monolayer-based switch exhibits a laser cooling effect, enabled by enhanced carrier excitation efficiency and prolonged carrier lifetimes, introducing a disruptive mechanism for laser cooling. Our findings highlight the strong potential of photodriven transient polaritons in advancing ultrafast thermal switches and nanoscale cooling technologies.

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Publication Details

Journal
ACS Nano
Published
2024-12-27
DOI
https://doi.org/10.1021/acsnano.4c14188
Citations
4
Primary Topic
Thermal Radiation and Cooling Technologies
Type
article
Field-Weighted Citation Impact
1.04

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article

Ultrafast Thermal Switching Enabled by Transient Polaritons

Bei Yang, Bai Song, F. Javier Garcı́a de Abajo, Qing Dai
4 citations
ACS Nano
Thermal Radiation and Cooling Technologies
1.04
article

Ultrafast Thermal Switching Enabled by Transient Polaritons

Bei Yang, Bai Song, F. Javier Garcı́a de Abajo, Qing Dai
article en
4 citations

Abstract

Ultrafast thermal switches are pivotal for managing heat generated in advanced solid-state applications, including high-speed chiplets, thermo-optical modulators, and on-chip lasers. However, conventional phonon-based switches cannot meet the demand for picosecond-level response times, and existing near-field radiative thermal switches face challenges in efficiently modulating heat transfer across vacuum gaps. To overcome these limitations, we propose an ultrafast thermal switch design based on pump-driven transient polaritons in asymmetric terminals. Demonstrated with WSe<sub>2</sub> and graphene, this approach achieves an impressive thermal switching ratio exceeding 10,000 with response times on the picosecond scale, outperforming current designs by at least 2 orders of magnitude. This exceptional performance is driven by dynamic polaritonic coupling between terminals, activated by ultrafast photoexcitation. Additionally, the WSe<sub>2</sub> monolayer-based switch exhibits a laser cooling effect, enabled by enhanced carrier excitation efficiency and prolonged carrier lifetimes, introducing a disruptive mechanism for laser cooling. Our findings highlight the strong potential of photodriven transient polaritons in advancing ultrafast thermal switches and nanoscale cooling technologies.

ACS NanoVol. 19(1)
Institució Catalana de Recerca i Estudis Avançats (ES), Institute of Photonic Sciences (ES), Shanghai Jiao Tong University (CN), Peking University (CN), Center for NanoScience (DE), Shanghai Institute for Science of Science (CN), Beijing Microelectronics Technology Institute (CN), Physical Measurement Laboratory (US), Barcelona Institute of Science and Technology (ES), National Center for Nanoscience and Technology (CN), University of Chinese Academy of Sciences (CN), Institute of Science and Technology
National Natural Science Foundation of China, Chinese Academy of Sciences, National Key Research and Development Program of China
Affordable and clean energy
Openalex Percentile: Top 24%
Thermal Radiation and Cooling Technologies
1.04
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