Phonon Inverse Faraday Effect from Electron-Phonon Coupling

The phonon inverse Faraday effect describes the emergence of a dc magnetization due to circularly polarized phonons. In this work we present a microscopic formalism for the phonon inverse Faraday effect. The formalism is based on time-dependent second order perturbation theory and electron phonon coupling. While our final equation is general and material independent, we provide estimates for the effective magnetic field expected for the ferroelectric soft mode in the oxide perovskite SrTiO_{3}. Our estimates are consistent with recent experiments showing a huge magnetization after a coherent excitation of circularly polarized phonons with THz laser light. Hence, the theoretical approach presented here is promising for shedding light into the microscopic mechanism of angular momentum transfer between ionic and electronic angular momentum, which is expected to play a central role in the phononic manipulation of magnetism.

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Publication Details

Journal
Physical Review Letters
Published
2024-12-26
DOI
https://doi.org/10.1103/physrevlett.133.266702
Citations
9
Primary Topic
Mechanical and Optical Resonators
Type
article
Field-Weighted Citation Impact
3.04

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article

Phonon Inverse Faraday Effect from Electron-Phonon Coupling

R. Matthias Geilhufe, Natalia Shabala
9 citations
Physical Review Letters
Mechanical and Optical Resonators
3.04
article

Phonon Inverse Faraday Effect from Electron-Phonon Coupling

R. Matthias Geilhufe, Natalia Shabala
article en
9 citations

Abstract

The phonon inverse Faraday effect describes the emergence of a dc magnetization due to circularly polarized phonons. In this work we present a microscopic formalism for the phonon inverse Faraday effect. The formalism is based on time-dependent second order perturbation theory and electron phonon coupling. While our final equation is general and material independent, we provide estimates for the effective magnetic field expected for the ferroelectric soft mode in the oxide perovskite SrTiO_{3}. Our estimates are consistent with recent experiments showing a huge magnetization after a coherent excitation of circularly polarized phonons with THz laser light. Hence, the theoretical approach presented here is promising for shedding light into the microscopic mechanism of angular momentum transfer between ionic and electronic angular momentum, which is expected to play a central role in the phononic manipulation of magnetism.

Physical Review LettersVol. 133(26)
Chalmers University of Technology (SE)
Chalmers Tekniska Högskola, Knut och Alice Wallenbergs Stiftelse, Stiftelsen Olle Engkvist Byggmästare, Vetenskapsrådet, Kungliga Fysiografiska Sällskapet i Lund, Wallenberg Center for Quantum Technology, Chalmers University of Technology
Openalex Percentile: Top 8%
Mechanical and Optical Resonators
3.04
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Phonon Inverse Faraday Effect from Electron-Phonon Coupling — R. Matthias Geilhufe, Natalia Shabala · Physical Review Letters (2024) | TGRS Research Map | TGRS