Enhancing Li-S Battery Performance with Porous Carbon from Hanji

Hanji-derived porous carbon has been developed and utilized as a cathode material for Li-S batteries, demonstrating exceptional electrochemical performance and stability. The unique porous structure and high surface area of Hanji-based carbon enhanced S utilization and significantly improved the overall efficiency of the battery. The material exhibited excellent electrical conductivity and structural stability, effectively addressing the major challenges of Li-S batteries, such as the polysulfide shuttle effect and active material loss. In addition, flake carbon-coated separators (FCCSs) were integrated into Li-S cells to further enhance their performance, achieving a high initial specific capacity of approximately 1200 mAh/g and maintaining a capacity of 620 mAh/g after 100 cycles. In contrast, cells with conventional polypropylene separators exhibited lower initial capacities (946 mAh/g), which decreased to 366 mAh/g after 100 cycles. FCCSs also demonstrated superior capacity retention and stability under varying charge–discharge rates, maintaining a capacity of 200 mAh/g at 3 C and recovering to 730 mAh/g when the rate was 0.1 C. This study provides valuable insights into the development of sustainable and efficient Li-S battery systems, with Hanji-based carbon and FCCSs emerging as promising components for commercial applications.

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Publication Details

Journal
Batteries
Published
2024-12-25
DOI
https://doi.org/10.3390/batteries11010004
Citations
3
Primary Topic
Advanced Battery Materials and Technologies
Type
article
Field-Weighted Citation Impact
0.63

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Enhancing Li-S Battery Performance with Porous Carbon from Hanji

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article

Enhancing Li-S Battery Performance with Porous Carbon from Hanji

Jong Pil Kim, Sei‐Jin Lee, Euh Duck Jeong, Yunju Choi, Heon‐Cheol Shin, Jong‐Seong Bae, Jae-Yeong Lee
article en
3 citations

Abstract

Hanji-derived porous carbon has been developed and utilized as a cathode material for Li-S batteries, demonstrating exceptional electrochemical performance and stability. The unique porous structure and high surface area of Hanji-based carbon enhanced S utilization and significantly improved the overall efficiency of the battery. The material exhibited excellent electrical conductivity and structural stability, effectively addressing the major challenges of Li-S batteries, such as the polysulfide shuttle effect and active material loss. In addition, flake carbon-coated separators (FCCSs) were integrated into Li-S cells to further enhance their performance, achieving a high initial specific capacity of approximately 1200 mAh/g and maintaining a capacity of 620 mAh/g after 100 cycles. In contrast, cells with conventional polypropylene separators exhibited lower initial capacities (946 mAh/g), which decreased to 366 mAh/g after 100 cycles. FCCSs also demonstrated superior capacity retention and stability under varying charge–discharge rates, maintaining a capacity of 200 mAh/g at 3 C and recovering to 730 mAh/g when the rate was 0.1 C. This study provides valuable insights into the development of sustainable and efficient Li-S battery systems, with Hanji-based carbon and FCCSs emerging as promising components for commercial applications.

BatteriesVol. 11(1)
Korea Basic Science Institute (KR), Pusan National University (KR), Jeonju University (KR)
Korea Basic Science Institute
Industry, innovation and infrastructure
Openalex Percentile: Top 30%
Advanced Battery Materials and Technologies
0.63
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