Data-driven feasibility study of VGF β-Ga2O3 growth under traveling magnetic fields

• A feasible furnace design was proposed for TMF-driven VGF-Ga 2 O 3 growth. • Upward TMF effectively flattens the solid–liquid interface. • Lorentz force density is predicted using a symbolic regression equation. • Lorentz force shows quadratic AC dependence, periodic phase shift, and asymmetric Gaussian with frequency. Numerical simulations were conducted to examine the impact of a traveling magnetic field on the vertical gradient freeze growth of β-Ga 2 O 3 crystals within a coated sapphire crucible under an argon-oxygen atmosphere. The research aimed to enhance β-Ga 2 O 3 crystal growth by achieving a flatter solid–liquid interface through the application of Lorentz forces generated by KRIST MAG ∼ ® heaters. Furthermore, the study sought to identify a coating material that is chemically resistant and has a minimal effect on the magnitude of the Lorentz force. To derive an equation that relates the Lorentz force with key growth parameters, we utilized SISSO, a machine learning technique combining symbolic regression and compressed sensing. The numerical results indicated that an upward traveling magnetic field significantly modifies the solid–liquid interface shape by counteracting buoyancy, enhancing vortex strength, and flattening the previously convex interface. The Pt-Rh alloy coating demonstrated minimal impact on the Lorentz force magnitude. Lorentz force exhibited a quadratic dependence on AC, periodic with a phase shift, and an asymmetric Gaussian profile with frequency. Compressed sensing, along with numerical data, produced a broadly applicable and interpretable equation for predicting Lorentz force values in the VGF growth setup, identifying phase shift as a crucial variable.

Authors

Publication Details

Journal
Journal of Crystal Growth
Published
2024-12-25
DOI
https://doi.org/10.1016/j.jcrysgro.2024.128049
Citations
2
Primary Topic
Ga2O3 and related materials
Type
article
Field-Weighted Citation Impact
0.24

Funders

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article

Data-driven feasibility study of VGF β-Ga2O3 growth under traveling magnetic fields

Milena Petković, Natasha Dropka, Gagan Kumar Chappa
2 citations
Journal of Crystal Growth
Ga2O3 and related materials
0.24
article

Data-driven feasibility study of VGF β-Ga2O3 growth under traveling magnetic fields

Milena Petković, Natasha Dropka, Gagan Kumar Chappa
article en
2 citations

Abstract

• A feasible furnace design was proposed for TMF-driven VGF-Ga 2 O 3 growth. • Upward TMF effectively flattens the solid–liquid interface. • Lorentz force density is predicted using a symbolic regression equation. • Lorentz force shows quadratic AC dependence, periodic phase shift, and asymmetric Gaussian with frequency. Numerical simulations were conducted to examine the impact of a traveling magnetic field on the vertical gradient freeze growth of β-Ga 2 O 3 crystals within a coated sapphire crucible under an argon-oxygen atmosphere. The research aimed to enhance β-Ga 2 O 3 crystal growth by achieving a flatter solid–liquid interface through the application of Lorentz forces generated by KRIST MAG ∼ ® heaters. Furthermore, the study sought to identify a coating material that is chemically resistant and has a minimal effect on the magnitude of the Lorentz force. To derive an equation that relates the Lorentz force with key growth parameters, we utilized SISSO, a machine learning technique combining symbolic regression and compressed sensing. The numerical results indicated that an upward traveling magnetic field significantly modifies the solid–liquid interface shape by counteracting buoyancy, enhancing vortex strength, and flattening the previously convex interface. The Pt-Rh alloy coating demonstrated minimal impact on the Lorentz force magnitude. Lorentz force exhibited a quadratic dependence on AC, periodic with a phase shift, and an asymmetric Gaussian profile with frequency. Compressed sensing, along with numerical data, produced a broadly applicable and interpretable equation for predicting Lorentz force values in the VGF growth setup, identifying phase shift as a crucial variable.

Journal of Crystal GrowthVol. 652
Deutsche Forschungsgemeinschaft, Forschungsverbund Berlin
Openalex Percentile: Top 55%
Ga2O3 and related materials
0.24
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