Electrical Contacts to Graphene by Postgrowth Patterning of Cu Foil for the Low-Cost Scalable Production of Graphene-Based Flexible Electronics

Numerous studies have focused on graphene owing to its potential as a next-generation electronic material, considering its high conductivity, transparency, superior mechanical stiffness, and flexibility. However, cost-effective mass production of graphene-based electronics based on existing fabrication methods, such as graphene transfer and metal formation, remains a challenge. This study proposes a simple and efficient method for creating electrical contacts with graphene. The method involves patterning a Cu foil after graphene growth, enabling the low-cost scalable production of graphene-based flexible electronics. The fabricated graphene devices exhibited linear current-voltage characteristics, indicating good electrical contact between the postgrowth-patterned Cu electrodes and graphene. The proposed postgrowth patterning method allows for the fabrication of Cu-contacted graphene devices on large areas and various flexible substrates, including ultrathin and stretchable films (<10 μm). The feasibility of the proposed method for electronic devices was demonstrated by implementing gas and flexible force sensors. The proposed approach advances the field of graphene-based electronics and holds potential for practical applications in various electronic devices, paving the way for scalable, cost-effective, and flexible technology solutions.