Photoinduced charge, spin, and orbital order in the two-orbital extended Hubbard model

Nonequilibrium control of electronically ordered hidden phases may lead to the development of ultrafast switches and memory devices. In this study, we demonstrate tunable hidden orders in the half-filled photodoped two-orbital extended Hubbard model. Using steady-state nonequilibrium dynamical mean-field theory, we clarify the coexistence and interplay of nonthermal charge, spin, and orbital order. The hidden state at low effective temperature and sufficiently high photodoping is reminiscent of Kugel-Khomskii order in the two-orbital Hubbard model at $\frac{1}{4}$ and $\frac{3}{4}$ filling, but it emerges out of a nonequilibrium charge-ordered state and exhibits a different magnetic structure. A low-energy effective Hamiltonian is used to analyze the exchange processes that stabilize the nonthermal order.

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Journal
Physical review. B./Physical review. B
Published
2024-12-20
DOI
https://doi.org/10.1103/physrevb.110.214433
Citations
1
Primary Topic
Physics of Superconductivity and Magnetism
Type
article
Field-Weighted Citation Impact
0.31

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article

Photoinduced charge, spin, and orbital order in the two-orbital extended Hubbard model

Sujay Ray, Philipp Werner
1 citations
Physical review. B./Physical review. B
Physics of Superconductivity and Magnetism
0.31
article

Photoinduced charge, spin, and orbital order in the two-orbital extended Hubbard model

Sujay Ray, Philipp Werner
article en
1 citations

Abstract

Nonequilibrium control of electronically ordered hidden phases may lead to the development of ultrafast switches and memory devices. In this study, we demonstrate tunable hidden orders in the half-filled photodoped two-orbital extended Hubbard model. Using steady-state nonequilibrium dynamical mean-field theory, we clarify the coexistence and interplay of nonthermal charge, spin, and orbital order. The hidden state at low effective temperature and sufficiently high photodoping is reminiscent of Kugel-Khomskii order in the two-orbital Hubbard model at $\frac{1}{4}$ and $\frac{3}{4}$ filling, but it emerges out of a nonequilibrium charge-ordered state and exhibits a different magnetic structure. A low-energy effective Hamiltonian is used to analyze the exchange processes that stabilize the nonthermal order.

Physical review. B./Physical review. BVol. 110(21)
University of Fribourg (CH)
Schweizerischer Nationalfonds zur Förderung der Wissenschaftlichen Forschung, Université de Fribourg
Openalex Percentile: Top 40%
Physics of Superconductivity and Magnetism
0.31
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