Ultrathin BIC Metasurfaces Based on Ultra-Low-Loss Sb<sub>2</sub>Se<sub>3</sub> Phase-Change Material

Ultrathin and low-loss phase-change materials (PCMs) are highly valued for their fast and effective phase transitions and applications in reconfigurable photonic chips, metasurfaces, optical modulators, sensors, photonic memories, and neuromorphic computing. However, conventional PCMs mostly suffer from high intrinsic losses in the near-infrared (NIR) region, limiting their potential for high quality factor (<i>Q</i>-factor) resonant metasurfaces. Here we present the design and fabrication of tunable bound states in the continuum (BIC) metasurfaces using the ultra-low-loss PCM Sb<sub>2</sub>Se<sub>3</sub>. Our BIC metasurfaces, only 25 nm thick, achieve high modulation depth and broad resonance tuning in the NIR with high <i>Q</i>-factors up to 130. Experimentally, we employ these BIC metasurfaces to modulate photoluminescence in rare earth-doped upconversion nanoparticles, reducing the excitation power for multiphoton photoluminescence and enabling emission polarization manipulation. This work offers a promising platform for developing active resonant metasurfaces, with broad applications including optical modulation, ultrafast switches, color filtering, and optical sensing.

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Publication Details

Journal
Nano Letters
Published
2024-12-19
DOI
https://doi.org/10.1021/acs.nanolett.4c04904
Citations
22
Primary Topic
Phase-change materials and chalcogenides
Type
article
Field-Weighted Citation Impact
2.58

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Ultrathin BIC Metasurfaces Based on Ultra-Low-Loss Sb2Se3 Phase-Change Material

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Ultrathin BIC Metasurfaces Based on Ultra-Low-Loss Sb2Se3 Phase-Change Material

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article en
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Abstract

Ultrathin and low-loss phase-change materials (PCMs) are highly valued for their fast and effective phase transitions and applications in reconfigurable photonic chips, metasurfaces, optical modulators, sensors, photonic memories, and neuromorphic computing. However, conventional PCMs mostly suffer from high intrinsic losses in the near-infrared (NIR) region, limiting their potential for high quality factor (<i>Q</i>-factor) resonant metasurfaces. Here we present the design and fabrication of tunable bound states in the continuum (BIC) metasurfaces using the ultra-low-loss PCM Sb<sub>2</sub>Se<sub>3</sub>. Our BIC metasurfaces, only 25 nm thick, achieve high modulation depth and broad resonance tuning in the NIR with high <i>Q</i>-factors up to 130. Experimentally, we employ these BIC metasurfaces to modulate photoluminescence in rare earth-doped upconversion nanoparticles, reducing the excitation power for multiphoton photoluminescence and enabling emission polarization manipulation. This work offers a promising platform for developing active resonant metasurfaces, with broad applications including optical modulation, ultrafast switches, color filtering, and optical sensing.

Nano LettersVol. 25(1)
University of Exeter (GB), ARC Centre of Excellence for Transformative Meta-Optical Systems (AU), Imperial College London (GB), Monash University (AU), RMIT University (AU), Macquarie University (AU)
Australian Research Council
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Openalex Percentile: Top 6%
Phase-change materials and chalcogenides
2.58
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