Optical and transport properties of NbN thin films revisited

Highly disordered NbN thin films exhibit promising superconducting and optical properties. Despite extensive study, discrepancies in its basic electronic properties persist. Analysis of the optical conductivity of disordered ultrathin NbN films, obtained from spectroscopic ellipsometry by the standard Drude-Lorentz model, provides inconsistent parameters. We argue that this discrepancy arises from neglecting the presence of quantum corrections to conductivity in the IR range. To resolve this matter, we suggest a modification to the Drude-Lorentz model, incorporating quantum corrections. The parameters obtained from the modified model are consistent with transport and superconducting measurements. The revisited values describing conduction electrons, which differ significantly from commonly adopted ones, are the electron relaxation rate $\mathrm{\ensuremath{\Gamma}}\ensuremath{\approx}1.8\phantom{\rule{4pt}{0ex}}\text{eV}/\ensuremath{\hbar}$, the Fermi velocity ${v}_{F}\ensuremath{\approx}0.7\ifmmode\times\else\texttimes\fi{}{10}^{6}\phantom{\rule{4pt}{0ex}}{\text{ms}}^{\ensuremath{-}1}$, and the electron density of states $N({E}_{F})=2\phantom{\rule{0.16em}{0ex}}$ states of both spins/eV/${V}_{\text{f.u.}}$.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2024-12-18
DOI
https://doi.org/10.1103/physrevb.110.245131
Citations
2
Primary Topic
Metal and Thin Film Mechanics
Type
article
Field-Weighted Citation Impact
0.54

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article

Optical and transport properties of NbN thin films revisited

T. Roch, Martin Baránek, Magdaléna Poláčková, P. Neilinger et al.
2 citations
Physical review. B./Physical review. B
Metal and Thin Film Mechanics
0.54
article

Optical and transport properties of NbN thin films revisited

T. Roch, Martin Baránek, Magdaléna Poláčková, P. Neilinger, Samuel Kern, M. Grajcar, T. Pleceník
article en
2 citations

Abstract

Highly disordered NbN thin films exhibit promising superconducting and optical properties. Despite extensive study, discrepancies in its basic electronic properties persist. Analysis of the optical conductivity of disordered ultrathin NbN films, obtained from spectroscopic ellipsometry by the standard Drude-Lorentz model, provides inconsistent parameters. We argue that this discrepancy arises from neglecting the presence of quantum corrections to conductivity in the IR range. To resolve this matter, we suggest a modification to the Drude-Lorentz model, incorporating quantum corrections. The parameters obtained from the modified model are consistent with transport and superconducting measurements. The revisited values describing conduction electrons, which differ significantly from commonly adopted ones, are the electron relaxation rate $\mathrm{\ensuremath{\Gamma}}\ensuremath{\approx}1.8\phantom{\rule{4pt}{0ex}}\text{eV}/\ensuremath{\hbar}$, the Fermi velocity ${v}_{F}\ensuremath{\approx}0.7\ifmmode\times\else\texttimes\fi{}{10}^{6}\phantom{\rule{4pt}{0ex}}{\text{ms}}^{\ensuremath{-}1}$, and the electron density of states $N({E}_{F})=2\phantom{\rule{0.16em}{0ex}}$ states of both spins/eV/${V}_{\text{f.u.}}$.

Physical review. B./Physical review. BVol. 110(24)
Slovak Academy of Sciences (SK), Comenius University Bratislava (SK)
European Commission, Agentúra na Podporu Výskumu a Vývoja, QuantERA, European Regional Development Fund
Openalex Percentile: Top 37%
Metal and Thin Film Mechanics
0.54
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