Thermal Rectification in Telescopic Nanowires: Impact of Thermal Boundary Resistance
A thermal diode, which, by analogy to its electrical counterpart, rectifies heat current, is the building block for thermal circuits. To realize a thermal diode, we demonstrate thermal rectification in a GaAs telescopic nanowire system using the thermal bridge method. We measured a preferred direction of heat flux, achieving rectification values ranging from 2 to 8% as a function of applied thermal bias. We demonstrate that the thermal boundary resistance between the thin part with the wurtzite crystal phase and the thick part with the zinc-blende crystal phase of the telescopic nanowire plays a crucial role in determining the amount and direction of heat flux rectification. This effect is confirmed by numerical solutions of the one-dimensional heat equation based on ab initio data. Additionally, we accounted for the effect of the thermal contact resistance. This work is the first experimental indication of rectification using a telescopic nanowire where we reveal the importance and role of the thermal boundary resistance in determining thermal rectification.
Authors
- Riccardo Rurali (ORCID: https://orcid.org/0000-0002-4086-4191)
- Saeko Tachikawa (ORCID: https://orcid.org/0000-0002-3752-0072)
- Anna Fontcuberta i Morral (ORCID: https://orcid.org/0000-0002-5070-2196)
- Milo Yaro Swinkels (ORCID: https://orcid.org/0000-0003-3710-2222)
- Miquel López-Suárez (ORCID: https://orcid.org/0000-0003-2338-277X)
- Yashpreet Kaur (ORCID: https://orcid.org/0009-0003-3762-3623)
- Alicia Ruiz‐Caridad (ORCID: https://orcid.org/0009-0001-4894-8322)
- Wonjong Kim (ORCID: https://orcid.org/0000-0001-6856-6607)
- Ilaria Zardo (ORCID: https://orcid.org/0000-0002-8685-2305)
- Matteo Camponovo
Institutions
- University of Basel (CH)
- Institut de Ciència de Materials de Barcelona (ES)
- Swiss Nanoscience Institute
- École Polytechnique Fédérale de Lausanne (CH)
Publication Details
- Journal
- ACS Applied Materials & Interfaces
- Published
- 2024-12-18
- DOI
- https://doi.org/10.1021/acsami.4c14920
- Citations
- 3
- Primary Topic
- Thermal properties of materials
- Type
- article
- Field-Weighted Citation Impact
- 0.35
Funders
- Ministerio de Ciencia, Innovación y Universidades
- Fundación Carmen y Severo Ochoa
- European Commission
- Generalitat de Catalunya
- Agencia Estatal de Investigación
- H2020 European Research Council