Tuning interfacial charge transport <i>via</i> Ti–O–Sn bonds for efficient CO<sub>2</sub> conversion
Here, the clever design of forming an ohmic contact between SnS<sub>2</sub> and MXene can regulate interfacial electron transport through Ti-O-Sn chemical bonds. This fast directional charge transport kinetics is attributed to the built-in electric field formed by the ohmic contact. As expected, the photoreduction CO<sub>2</sub> activity of the optimized SSTC-5 catalyst is 10.4 times that of the original SnS<sub>2</sub>.
Authors
- Pengwei Huo (ORCID: https://orcid.org/0000-0001-9899-0820)
- Yiying Zhou
- Binrong Li (ORCID: https://orcid.org/0000-0003-3496-8362)
- Yingying Qin (ORCID: https://orcid.org/0000-0002-6716-8401)
- Shikang Yin (ORCID: https://orcid.org/0000-0001-9647-7871)
- F.Y. Zhou (ORCID: https://orcid.org/0009-0004-9392-8816)
- Yuming Sun (ORCID: https://orcid.org/0000-0001-7790-2641)
- Yan Yan (ORCID: https://orcid.org/0000-0003-2393-3017)
Institutions
- Jiangsu University (CN)
- Hong Kong Polytechnic University (HK)
- Suzhou University of Science and Technology (CN)
Publication Details
- Journal
- Chemical Communications
- Published
- 2024-12-18
- DOI
- https://doi.org/10.1039/d4cc05929h
- Citations
- 2
- Primary Topic
- Advanced Photocatalysis Techniques
- Type
- article
- Field-Weighted Citation Impact
- 0.20
Funders
- National Natural Science Foundation of China