Probing quantum geometry through optical conductivity and magnetic circular dichroism
Probing ground-state quantum geometry and topology through optical responses is not only of fundamental interest, but it can also offer several practical advantages. Here, using first-principles calculations on thin films of the antiferromagnetic topological insulator MnBi<sub>2</sub>Te<sub>4</sub>, we demonstrate how the generalized optical weight arising from the absorptive part of the optical conductivity can be used to probe the ground-state quantum geometry and topology. We show that three-septuple-layer MnBi<sub>2</sub>Te<sub>4</sub> film exhibit an enhanced, almost-perfect magnetic circular dichroism for a narrow photon energy window in the infrared region. We calculate the quantum weight in this MnBi<sub>2</sub>Te<sub>4</sub> film and show that it far exceeds the lower bound provided by the Chern number. Our results suggest that the well-known optical methods are powerful tools for probing the ground-state quantum geometry and topology.
Authors
- Hsin Lin (ORCID: https://orcid.org/0000-0002-4688-2315)
- Su‐Yang Xu (ORCID: https://orcid.org/0009-0006-6819-3613)
- Barun Ghosh (ORCID: https://orcid.org/0000-0001-6634-0508)
- Yugo Onishi (ORCID: https://orcid.org/0000-0003-0004-6124)
- Arun Bansil (ORCID: https://orcid.org/0000-0002-3864-3461)
- Liang Fu (ORCID: https://orcid.org/0000-0002-8803-1017)
Institutions
- Northeastern University (US)
- Harvard University (US)
- Institute of Physics, Academia Sinica (TW)
- Eastern University (BD)
- Massachusetts Institute of Technology (US)
Publication Details
- Journal
- Science Advances
- Published
- 2024-12-18
- DOI
- https://doi.org/10.1126/sciadv.ado1761
- Citations
- 23
- Primary Topic
- Topological Materials and Phenomena
- Type
- article
- Field-Weighted Citation Impact
- 7.76