Probing quantum geometry through optical conductivity and magnetic circular dichroism

Probing ground-state quantum geometry and topology through optical responses is not only of fundamental interest, but it can also offer several practical advantages. Here, using first-principles calculations on thin films of the antiferromagnetic topological insulator MnBi<sub>2</sub>Te<sub>4</sub>, we demonstrate how the generalized optical weight arising from the absorptive part of the optical conductivity can be used to probe the ground-state quantum geometry and topology. We show that three-septuple-layer MnBi<sub>2</sub>Te<sub>4</sub> film exhibit an enhanced, almost-perfect magnetic circular dichroism for a narrow photon energy window in the infrared region. We calculate the quantum weight in this MnBi<sub>2</sub>Te<sub>4</sub> film and show that it far exceeds the lower bound provided by the Chern number. Our results suggest that the well-known optical methods are powerful tools for probing the ground-state quantum geometry and topology.

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Publication Details

Journal
Science Advances
Published
2024-12-18
DOI
https://doi.org/10.1126/sciadv.ado1761
Citations
23
Primary Topic
Topological Materials and Phenomena
Type
article
Field-Weighted Citation Impact
7.76
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article

Probing quantum geometry through optical conductivity and magnetic circular dichroism

Hsin Lin, Su‐Yang Xu, Barun Ghosh, Yugo Onishi et al.
23 citations
Science Advances
Topological Materials and Phenomena
7.76
article

Probing quantum geometry through optical conductivity and magnetic circular dichroism

Hsin Lin, Su‐Yang Xu, Barun Ghosh, Yugo Onishi, Arun Bansil, Liang Fu
article en
23 citations

Abstract

Probing ground-state quantum geometry and topology through optical responses is not only of fundamental interest, but it can also offer several practical advantages. Here, using first-principles calculations on thin films of the antiferromagnetic topological insulator MnBi<sub>2</sub>Te<sub>4</sub>, we demonstrate how the generalized optical weight arising from the absorptive part of the optical conductivity can be used to probe the ground-state quantum geometry and topology. We show that three-septuple-layer MnBi<sub>2</sub>Te<sub>4</sub> film exhibit an enhanced, almost-perfect magnetic circular dichroism for a narrow photon energy window in the infrared region. We calculate the quantum weight in this MnBi<sub>2</sub>Te<sub>4</sub> film and show that it far exceeds the lower bound provided by the Chern number. Our results suggest that the well-known optical methods are powerful tools for probing the ground-state quantum geometry and topology.

Science AdvancesVol. 10(51)
Northeastern University (US), Harvard University (US), Institute of Physics, Academia Sinica (TW), Eastern University (BD), Massachusetts Institute of Technology (US)
Affordable and clean energy
Openalex Percentile: Top 2%
Topological Materials and Phenomena
7.76
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