Magnetic and Electronic Inhomogeneity in Sm1−xEuxB6

While SmB6 attracts attention as a possible topological Kondo insulator, EuB6 is known to host magnetic polarons that give rise to large magnetoresistive effects above its ferromagnetic order transition. Here, we investigate single crystals of Sm1−xEuxB6 by magnetic and magnetotransport measurements to explore a possible interplay of these two intriguing phenomena, with a focus on the Eu-rich substitutions. Sm0.01Eu0.99B6 exhibits generally similar behavior as EuB6. Interestingly, Sm0.05Eu0.95B6 combines a global antiferromagnetic order with local polaron formation. A pronounced hysteresis is found in the magnetoresistance of Sm0.1Eu0.9B6 at low temperature (T= 1.9 K) and applied magnetic fields between 2.3 and 3.6 T. The latter is in agreement with a phenomenological model that predicts the stabilization of ferromagnetic polarons with an increasing magnetic field within materials with a global antiferromagnetic order.

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Publication Details

Journal
Condensed Matter
Published
2024-12-13
DOI
https://doi.org/10.3390/condmat9040055
Primary Topic
Rare-earth and actinide compounds
Type
article
Field-Weighted Citation Impact
0.00

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article

Magnetic and Electronic Inhomogeneity in Sm1−xEuxB6

S. Wirth, P. Schlottmann, Jens Müller, M. Victoria Ale Crivillero et al.
Condensed Matter
Rare-earth and actinide compounds
article

Magnetic and Electronic Inhomogeneity in Sm1−xEuxB6

S. Wirth, P. Schlottmann, Jens Müller, M. Victoria Ale Crivillero, P. F. S. Rosa, Z. Fisk
article en

Abstract

While SmB6 attracts attention as a possible topological Kondo insulator, EuB6 is known to host magnetic polarons that give rise to large magnetoresistive effects above its ferromagnetic order transition. Here, we investigate single crystals of Sm1−xEuxB6 by magnetic and magnetotransport measurements to explore a possible interplay of these two intriguing phenomena, with a focus on the Eu-rich substitutions. Sm0.01Eu0.99B6 exhibits generally similar behavior as EuB6. Interestingly, Sm0.05Eu0.95B6 combines a global antiferromagnetic order with local polaron formation. A pronounced hysteresis is found in the magnetoresistance of Sm0.1Eu0.9B6 at low temperature (T= 1.9 K) and applied magnetic fields between 2.3 and 3.6 T. The latter is in agreement with a phenomenological model that predicts the stabilization of ferromagnetic polarons with an increasing magnetic field within materials with a global antiferromagnetic order.

Condensed MatterVol. 9(4)
Florida State University (US), Goethe University Frankfurt (DE), Los Alamos National Laboratory (US), University of California, Irvine (US), Max Planck Institute for Chemical Physics of Solids (DE)
Deutsche Forschungsgemeinschaft
Openalex Percentile: Top 86%
Rare-earth and actinide compounds
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