One-Step Construction of Atropisomers Bearing 1,5-Central and Axial Chirality via Catalytic Diastereo- and Atroposelective Remote Desymmetrizing Alkynylation

Catalytic asymmetric construction of atropisomers with multiple stereogenic elements has recently become an emerging area. However, general methods that produced atropisomers bearing remote 1,5-axial and central chirality efficiently and stereoselectively are scarce yet highly challenging. We herein report a catalytic diastereo- and atroposelective remote desymmetrizing alkynylation of axially prochiral dialkynes with ortho-quinone methides (o-QMs), furnishing atropisomers bearing 1,5-remote centrally and axially stereogenic elements. The remote control of prochiral axis far from the reaction site could be simultaneously achieved during the stereoselective C(sp3)–C(sp) bond-forming process to generate a stereogenic center. In addition, a kinetic resolution of axially racemic alkynes via diastereo- and atroposelective remote alkynylation with o-QMs has been developed, further enriching structural diversity of atropisomers bearing 1,5-central and axial chirality. The present method expands the chemical space of atropisomeric molecules bearing multiple chiral elements by facile downstream diversification of C–C triple bonds. Finally, the alkynylation of o-QMs can also be applied for the construction of chiral motifs bearing 1,9- and 1,10-stereogenic centers.

Authors

Institutions

Publication Details

Journal
ACS Catalysis
Published
2024-12-12
DOI
https://doi.org/10.1021/acscatal.4c06332
Citations
7
Primary Topic
Axial and Atropisomeric Chirality Synthesis
Type
article
Field-Weighted Citation Impact
1.75

Funders

Controls
|||
ALL TIME
JAN
FEB
MAR
APR
MAY
JUN
JUL
AUG
SEP
OCT
article

One-Step Construction of Atropisomers Bearing 1,5-Central and Axial Chirality via Catalytic Diastereo- and Atroposelective Remote Desymmetrizing Alkynylation

Fangzhi Peng, Kaixin Zhao, Zhihui Shao, Ming Jiang et al.
7 citations
ACS Catalysis
Axial and Atropisomeric Chirality Synthesis
1.75
article

One-Step Construction of Atropisomers Bearing 1,5-Central and Axial Chirality via Catalytic Diastereo- and Atroposelective Remote Desymmetrizing Alkynylation

Fangzhi Peng, Kaixin Zhao, Zhihui Shao, Ming Jiang, Yingcheng Wang, Xiaoguang Li, Shan Wang, Zheng Wang, Long Li, Daming He
article en
7 citations

Abstract

Catalytic asymmetric construction of atropisomers with multiple stereogenic elements has recently become an emerging area. However, general methods that produced atropisomers bearing remote 1,5-axial and central chirality efficiently and stereoselectively are scarce yet highly challenging. We herein report a catalytic diastereo- and atroposelective remote desymmetrizing alkynylation of axially prochiral dialkynes with ortho-quinone methides (o-QMs), furnishing atropisomers bearing 1,5-remote centrally and axially stereogenic elements. The remote control of prochiral axis far from the reaction site could be simultaneously achieved during the stereoselective C(sp3)–C(sp) bond-forming process to generate a stereogenic center. In addition, a kinetic resolution of axially racemic alkynes via diastereo- and atroposelective remote alkynylation with o-QMs has been developed, further enriching structural diversity of atropisomers bearing 1,5-central and axial chirality. The present method expands the chemical space of atropisomeric molecules bearing multiple chiral elements by facile downstream diversification of C–C triple bonds. Finally, the alkynylation of o-QMs can also be applied for the construction of chiral motifs bearing 1,9- and 1,10-stereogenic centers.

ACS CatalysisVol. 14(24)
Shenzhen University (CN), Yunnan University (CN)
National Natural Science Foundation of China, Major Science and Technology Projects in Yunnan Province
Openalex Percentile: Top 16%
Axial and Atropisomeric Chirality Synthesis
1.75
AI Navigator

Ask Laika to Summarize, Analyze, and Connect papers live on the map.

Summarize Papers & Methodologies

Extract key findings, datasets, and comparative methods across publications.

Benchmark Rankings & Visual Analytics

Rank top research institutions, authors, funders, topics, and journals by Field-Weighted Citation Impact (FWCI) and paper volume with instant charts.

Connect Distant Disciplines

Bridge topological clusters on the map to find hidden collaborative intersections.