Ice-nucleating particle concentration impacts cloud properties over Dronning Maud Land, East Antarctica, in COSMO-CLM <sup>2</sup>

Abstract. Ice-nucleating particles (INPs) have an important function in the freezing of clouds but are rare in East Antarctica. At the Belgian Princess Elisabeth Antarctica station, immersion freezing INP concentrations between 6×10-6 and 5×10-3 L−1 have been observed with an activation temperature of −20 °C. These low concentrations offer a possible explanation for the occurrence of supercooled liquid water in clouds observed using the station's micro rain radar and ceilometer. We used the model of the Consortium for Small-scale Modeling (COSMO) in climate mode (CLM) coupled to the Community Land Model (CLM) (COSMO-CLM2) with an added aerosol-cycle module to test the cloud phase's sensitivity in response to varying prescribed INP concentrations. We tested two cases, one in austral summer and one in austral winter, and analysed the differences resulting from INP concentration changes for an area around the station and over the Southern Ocean within the selected domain. Our results show a strong influence of the INP concentration on the liquid water path in both regions, with higher concentrations reducing the amount of liquid water. Over the Southern Ocean, this effect is stronger during winter: during summer, a significant portion of water remains in liquid state regardless of INP concentration. Over the continent, this effect is stronger during summer: temperatures in winter frequently fall below −37 °C, allowing homogeneous freezing. The largest increase in the liquid water fraction of total cloud hydrometeor mass is simulated over the Southern Ocean in winter, from 9.8 % in the highest tested INP concentration to 50.3 % in the lowest. The radiative effects caused by the INP concentration changes are small, with less than 3 W m−2 difference in the averages between different concentrations.

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Publication Details

Journal
Atmospheric chemistry and physics
Published
2024-12-12
DOI
https://doi.org/10.5194/acp-24-13751-2024
Citations
1
Primary Topic
Atmospheric aerosols and clouds
Type
article
Field-Weighted Citation Impact
0.28

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article

Ice-nucleating particle concentration impacts cloud properties over Dronning Maud Land, East Antarctica, in COSMO-CLM 2

Nicole Van Lipzig, Alexander Mangold, Niels Souverijns, Florian Sauerland et al.
1 citations
Atmospheric chemistry and physics
Atmospheric aerosols and clouds
0.28
article

Ice-nucleating particle concentration impacts cloud properties over Dronning Maud Land, East Antarctica, in COSMO-CLM 2

Nicole Van Lipzig, Alexander Mangold, Niels Souverijns, Florian Sauerland, Anna Possner, Kwinten Van Weverberg, Preben Van Overmeiren, Heike Wex
article en
1 citations

Abstract

Abstract. Ice-nucleating particles (INPs) have an important function in the freezing of clouds but are rare in East Antarctica. At the Belgian Princess Elisabeth Antarctica station, immersion freezing INP concentrations between 6×10-6 and 5×10-3 L−1 have been observed with an activation temperature of −20 °C. These low concentrations offer a possible explanation for the occurrence of supercooled liquid water in clouds observed using the station's micro rain radar and ceilometer. We used the model of the Consortium for Small-scale Modeling (COSMO) in climate mode (CLM) coupled to the Community Land Model (CLM) (COSMO-CLM2) with an added aerosol-cycle module to test the cloud phase's sensitivity in response to varying prescribed INP concentrations. We tested two cases, one in austral summer and one in austral winter, and analysed the differences resulting from INP concentration changes for an area around the station and over the Southern Ocean within the selected domain. Our results show a strong influence of the INP concentration on the liquid water path in both regions, with higher concentrations reducing the amount of liquid water. Over the Southern Ocean, this effect is stronger during winter: during summer, a significant portion of water remains in liquid state regardless of INP concentration. Over the continent, this effect is stronger during summer: temperatures in winter frequently fall below −37 °C, allowing homogeneous freezing. The largest increase in the liquid water fraction of total cloud hydrometeor mass is simulated over the Southern Ocean in winter, from 9.8 % in the highest tested INP concentration to 50.3 % in the lowest. The radiative effects caused by the INP concentration changes are small, with less than 3 W m−2 difference in the averages between different concentrations.

Atmospheric chemistry and physicsVol. 24(23)
Royal Meteorological Institute of Belgium (BE), Goethe University Frankfurt (DE), Frankfurt Institute for Advanced Studies (DE), Ghent University (BE), Leibniz Institute for Tropospheric Research (DE), Flemish Institute for Technological Research (BE), KU Leuven (BE)
Vlaams Supercomputer Centrum, Belgian Federal Science Policy Office, Fonds Wetenschappelijk Onderzoek, Vlaamse regering
Life below water
Openalex Percentile: Top 40%
Atmospheric aerosols and clouds
0.28
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