Superconductivity from Domain Wall Fluctuations in Sliding Ferroelectrics

Bilayers of two-dimensional van der Waals materials that lack an inversion center can show a novel form of ferroelectricity, where certain stacking arrangements of the two layers lead to an interlayer polarization. Under an external out-of-plane electric field, a relative sliding between the two layers can occur, accompanied by an interlayer charge transfer and a ferroelectric switching. We show that the domain walls that mediate ferroelectric switching are a locus of strong attractive interactions between electrons. The attraction is mediated by the ferroelectric domain wall fluctuations, effectively driven by the soft interlayer shear phonon. We comment on the possible relevance of this attraction mechanism to the recent observation of an interplay between sliding ferroelectricity and superconductivity in bilayer T_{d}-MoTe_{2}. We also discuss the possible role of this mechanism in the superconductivity of moiré bilayers.

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Publication Details

Journal
Physical Review Letters
Published
2024-12-10
DOI
https://doi.org/10.1103/physrevlett.133.246001
Citations
4
Primary Topic
Electronic and Structural Properties of Oxides
Type
article
Field-Weighted Citation Impact
0.47

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article

Superconductivity from Domain Wall Fluctuations in Sliding Ferroelectrics

Gaurav Chaudhary, Ivar Martin
4 citations
Physical Review Letters
Electronic and Structural Properties of Oxides
0.47
article

Superconductivity from Domain Wall Fluctuations in Sliding Ferroelectrics

Gaurav Chaudhary, Ivar Martin
article en
4 citations

Abstract

Bilayers of two-dimensional van der Waals materials that lack an inversion center can show a novel form of ferroelectricity, where certain stacking arrangements of the two layers lead to an interlayer polarization. Under an external out-of-plane electric field, a relative sliding between the two layers can occur, accompanied by an interlayer charge transfer and a ferroelectric switching. We show that the domain walls that mediate ferroelectric switching are a locus of strong attractive interactions between electrons. The attraction is mediated by the ferroelectric domain wall fluctuations, effectively driven by the soft interlayer shear phonon. We comment on the possible relevance of this attraction mechanism to the recent observation of an interplay between sliding ferroelectricity and superconductivity in bilayer T_{d}-MoTe_{2}. We also discuss the possible role of this mechanism in the superconductivity of moiré bilayers.

Physical Review LettersVol. 133(24)
Argonne National Laboratory (US), University of Cambridge (GB)
U.S. Department of Energy, Office of Science, Basic Energy Sciences
Openalex Percentile: Top 37%
Electronic and Structural Properties of Oxides
0.47
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Superconductivity from Domain Wall Fluctuations in Sliding Ferroelectrics — Gaurav Chaudhary, Ivar Martin · Physical Review Letters (2024) | TGRS Research Map | TGRS