Polariton-Induced Transparency in Multiple Quantum Wells Probed by Time Domain Brillouin Scattering

The interference of the incident light reflected from the surface of a medium and from a picosecond strain pulse propagating through it results in temporal oscillations of the reflected intensity. This phenomenon, called time-domain Brillouin scattering, enables us to gain information about the optical field inside the medium. The oscillation amplitude decreases with increase of the distance from the strain pulse to the surface if the incident light is strongly absorbed, while it remains constant if the medium is transparent. Here we exploit time domain Brillouin scattering to probe the optical field inside a multiple quantum well layer for light strongly coupling to excitons and forming polaritons. At low excitation density, we observe conventional Brillouin oscillations whose amplitude is small when the strain pulse is positioned far from the surface due to the strong absorption of polaritons in the vicinity of the exciton resonance. At elevated optical density, the absorption disappears, the medium becomes transparent, and the amplitude of the oscillations does not depend on the distance of the strain pulse from the surface. We explain this effect of polariton-induced transparency by the increase of the incoherent exciton density generated as result of polariton scattering. Finally, the increase of the exciton density leads to transition of the exciton gas to a collective state, resulting in collapse of the polariton state and propagation of the incident light in the medium without absorption.

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Publication Details

Journal
ACS Photonics
Published
2024-12-10
DOI
https://doi.org/10.1021/acsphotonics.4c01357
Citations
1
Primary Topic
Mechanical and Optical Resonators
Type
article
Field-Weighted Citation Impact
0.34

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article

Polariton-Induced Transparency in Multiple Quantum Wells Probed by Time Domain Brillouin Scattering

A. K. Samusev, Mario Littmann, M. Bayer, А. В. Акимов et al.
1 citations
ACS Photonics
Mechanical and Optical Resonators
0.34
article

Polariton-Induced Transparency in Multiple Quantum Wells Probed by Time Domain Brillouin Scattering

A. K. Samusev, Mario Littmann, M. Bayer, А. В. Акимов, Marek Karzel, D. Reuter, A. V. Scherbakov, T. L. Linnik
article en
1 citations

Abstract

The interference of the incident light reflected from the surface of a medium and from a picosecond strain pulse propagating through it results in temporal oscillations of the reflected intensity. This phenomenon, called time-domain Brillouin scattering, enables us to gain information about the optical field inside the medium. The oscillation amplitude decreases with increase of the distance from the strain pulse to the surface if the incident light is strongly absorbed, while it remains constant if the medium is transparent. Here we exploit time domain Brillouin scattering to probe the optical field inside a multiple quantum well layer for light strongly coupling to excitons and forming polaritons. At low excitation density, we observe conventional Brillouin oscillations whose amplitude is small when the strain pulse is positioned far from the surface due to the strong absorption of polaritons in the vicinity of the exciton resonance. At elevated optical density, the absorption disappears, the medium becomes transparent, and the amplitude of the oscillations does not depend on the distance of the strain pulse from the surface. We explain this effect of polariton-induced transparency by the increase of the incoherent exciton density generated as result of polariton scattering. Finally, the increase of the exciton density leads to transition of the exciton gas to a collective state, resulting in collapse of the polariton state and propagation of the incident light in the medium without absorption.

ACS PhotonicsVol. 11(12)
University of Nottingham (GB), TU Dortmund University (DE), Paderborn University (DE), V.E. Lashkaryov Institute of Semiconductor Physics (UA)
Alexander von Humboldt-Stiftung, Deutsche Forschungsgemeinschaft, Universitätsallianz Ruhr, Technische Universität Dortmund
Decent work and economic growth
Openalex Percentile: Top 38%
Mechanical and Optical Resonators
0.34
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