Sign‐Switchable Poisson's Ratio Design for Bimodal Strain‐to‐Electrical Signal Transducing Device

Stretchable electronic devices that conduct strain-related electronic performances have drawn extensive attention, functioning as mechanical sensors, actuators, and stretchable conductors. Although strain-insensitive or strain-responsive nature is well-achieved separately, it remains challenging to combine these two characteristics in one single device, which will offer versatile adaptability in various working situations. Herein, a hybrid material with sign-switchable Poisson's ratio (SSPR) is developed by combining a phase-change gel based reentrantreentrant honeycomb pattern and a polydimethylsiloxane film. The phase-change gel featuring thermally-regulated Young's modulus enables the hybrid material to switch between negative and positive Poisson's ratios. After integrating with a pre-stretched silver nanowires film, the obtained stretchable device performs bimodal strain-to-electrical signal transducing (Bi-SET) functions, in which the SSPR-dominated strain-resistance response switches between strain-dependent and strain-insensitive behaviors. As a proof of concept, a mode-switchable grasping system is constructed using a Bi-SET device-based controller, enabling the adaptation of grasping behaviors to various target objects.