Anisotropy of the zigzag order in the Kitaev honeycomb magnet <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:mi>α</mml:mi><mml:mtext>−</mml:mtext><mml:msub><mml:mi>RuBr</mml:mi><mml:mn>3</mml:mn></mml:msub></mml:mrow></mml:ma

Kitaev materials often order magnetically at low temperatures due to the presence of non-Kitaev interactions. Torque magnetometry is a very sensitive technique for probing the magnetic anisotropy, which is critical in understanding the magnetic ground state. In this paper, we report detailed single-crystal torque measurements in the proposed Kitaev candidate honeycomb magnet <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"><a:mrow><a:mi>α</a:mi><a:mtext>−</a:mtext><a:msub><a:mi>RuBr</a:mi><a:mn>3</a:mn></a:msub></a:mrow></a:math>, which displays zigzag order below 34 K. Based on angular-dependent torque studies in magnetic fields up to 16 T rotated in the plane normal to the honeycomb layers, we find an easy-plane anisotropy with a temperature dependence of the torque amplitude following closely the behavior of the powder magnetic susceptibility. The torque for the field rotated in the honeycomb plane has a clear sixfold periodicity with a sawtooth shape, reflecting the threefold symmetry of the crystal structure and stabilization of different zigzag domains depending on the field orientation, with a torque amplitude that follows an order parameter form inside the zigzag phase. By comparing experimental data with theoretical calculations we highlight the importance of relevant anisotropic interactions and the role of the competition between different zigzag domains in this candidate Kitaev magnet. Published by the American Physical Society 2024

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2024-12-03
DOI
https://doi.org/10.1103/physrevb.110.214404
Citations
4
Primary Topic
Advanced Condensed Matter Physics
Type
article
Field-Weighted Citation Impact
1.24

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article

Anisotropy of the zigzag order in the Kitaev honeycomb magnet <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:mi>α</mml:mi><mml:mtext>−</mml:mtext><mml:msub><mml:mi>RuBr</mml:mi><mml:mn>3</mml:mn></mml:msub></mml:mrow></mml:ma

A. I. Coldea, R. Coldea, R. J. Cava, Danrui Ni et al.
4 citations
Physical review. B./Physical review. B
Advanced Condensed Matter Physics
1.24
article

Anisotropy of the zigzag order in the Kitaev honeycomb magnet <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:mi>α</mml:mi><mml:mtext>−</mml:mtext><mml:msub><mml:mi>RuBr</mml:mi><mml:mn>3</mml:mn></mml:msub></mml:mrow></mml:ma

A. I. Coldea, R. Coldea, R. J. Cava, Danrui Ni, Roser Valentí, David A. S. Kaib, Zeyu Ma, John S. Pearce
article en
4 citations

Abstract

Kitaev materials often order magnetically at low temperatures due to the presence of non-Kitaev interactions. Torque magnetometry is a very sensitive technique for probing the magnetic anisotropy, which is critical in understanding the magnetic ground state. In this paper, we report detailed single-crystal torque measurements in the proposed Kitaev candidate honeycomb magnet <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"><a:mrow><a:mi>α</a:mi><a:mtext>−</a:mtext><a:msub><a:mi>RuBr</a:mi><a:mn>3</a:mn></a:msub></a:mrow></a:math>, which displays zigzag order below 34 K. Based on angular-dependent torque studies in magnetic fields up to 16 T rotated in the plane normal to the honeycomb layers, we find an easy-plane anisotropy with a temperature dependence of the torque amplitude following closely the behavior of the powder magnetic susceptibility. The torque for the field rotated in the honeycomb plane has a clear sixfold periodicity with a sawtooth shape, reflecting the threefold symmetry of the crystal structure and stabilization of different zigzag domains depending on the field orientation, with a torque amplitude that follows an order parameter form inside the zigzag phase. By comparing experimental data with theoretical calculations we highlight the importance of relevant anisotropic interactions and the role of the competition between different zigzag domains in this candidate Kitaev magnet. Published by the American Physical Society 2024

Physical review. B./Physical review. BVol. 110(21)
Goethe University Frankfurt (DE), Princeton University (US), University of Oxford (GB)
National Science Foundation, Gordon and Betty Moore Foundation, University of Oxford, Deutsche Forschungsgemeinschaft, Engineering and Physical Sciences Research Council, Horizon 2020
Openalex Percentile: Top 20%
Advanced Condensed Matter Physics
1.24
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