High‐Performance Broad‐Spectrum UV Photodetectors with Uniform Response: Engineering β‐Ga <sub>2</sub> O <sub>3</sub> :Si/GaN:Si Heterojunctions via Thermal Oxidation for Optoelectronic Logic Gate and Multispectral Imaging
Developing high-performance, broad-spectrum ultraviolet photodetectors (PDs) with uniform response is crucial for optoelectronic applications like spectral analysis, optoelectronic logic gates, and multispectral imaging. This study constructs n-n type β-Ga<sub>2</sub>O<sub>3</sub>:Si/GaN:Si heterojunction PDs using thermal oxidation, combining the advantages of β-Ga<sub>2</sub>O<sub>3</sub>:Si and GaN:Si for excellent broad-spectrum response (UV-A to UV-C). A proposed channel model for GaN:Si oxidation includes hole formation, vortex structure development, channel formation, and grain growth, providing a basis for understanding β-Ga<sub>2</sub>O<sub>3</sub>:Si/GaN:Si heterojunction formation. Uniform Si doping in the β-Ga<sub>2</sub>O<sub>3</sub> layer, achieved through thermal oxidation, reduces resistivity, enhances the collection of photogenerated carriers from the underlying GaN layer, and hence enhances broad-spectrum response performance. The devices exhibit outstanding uniformity and sensitivity across the UV-A to UV-C range, with a peak responsivity of 2.44 × 10<sup>4</sup> A W<sup>-1</sup> and a photocurrent-to-dark current ratio of 1.3 × 10<sup>5</sup>. Applications include optoelectronic logic gates executing "OR gate" and "AND gate" logic operations with 254 and 365 nm UV light, and a single-pixel multispectral imaging system producing high-contrast, clear "CNU" images with 254, 295, and 365 nm UV light. This research advances the understanding of oxide heterojunction formation and offers a method for developing high-performance, uniformly responsive broad-spectrum UV photodetectors for optoelectronic applications.
Authors
- Ke Ding (ORCID: https://orcid.org/0009-0005-2846-8590)
- Wanjun Li (ORCID: https://orcid.org/0000-0003-4707-4288)
- Jiangshuai Luo
- Yan Tang (ORCID: https://orcid.org/0000-0002-3109-6987)
- Lijuan Ye (ORCID: https://orcid.org/0000-0001-9652-6311)
- Hong Zhang (ORCID: https://orcid.org/0000-0002-0868-9477)
- Jili Jiang
- Di Pang (ORCID: https://orcid.org/0009-0009-5969-0775)
Institutions
- Chongqing Normal University (CN)
Publication Details
- Journal
- Small
- Published
- 2024-12-01
- DOI
- https://doi.org/10.1002/smll.202406447
- Citations
- 30
- Primary Topic
- Ga2O3 and related materials
- Type
- article
- Field-Weighted Citation Impact
- 3.54
Funders
- National Natural Science Foundation of China
- Natural Science Foundation of Chongqing