Illumination conditions of photocatalyst-containing mist on the degradation of organic compounds

• The illumination conditions of photocatalyst-containing mist were studied. • UV light, ultrasound, and mist were applied to a mixture of TiO 2 and phenol. • Higher light intensities provided to the mist improved phenol degradation. • Excess TiO 2 prevented mist generation and utilization. • Findings inform the design of reactors that use photocatalysts and mist. Photocatalysis is a promising method for treating wastewater containing toxic organic pollutants. To improve the degradation of those pollutants, the utilization of mist that contains photocatalysts has been considered. In this study, the light illumination conditions of the mist that affect photocatalytic degradation were investigated to provide insight into the design of reactors that utilize photocatalyst-containing mist. In the reactor, UV light, ultrasound (US), and US-generated mist were applied to a mixture containing the TiO 2 photocatalyst and phenol as the model organic pollutant. The results indicated that higher UV intensities and TiO 2 dosages affected the illumination conditions to improve the degradation of phenol. However, at higher TiO 2 dosages, mist was not generated, so its enhanced illumination was not utilized in the degradation reactions. The analysis of the reaction kinetics suggested the enhancement of the illumination condition by the mist. These findings provide insight into the design of the reactor that utilizes photocatalyst-containing mist to improve the irradiation conditions and promote photocatalytic reactions.

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Publication Details

Journal
Chemical Engineering and Processing - Process Intensification
Published
2024-12-01
DOI
https://doi.org/10.1016/j.cep.2024.110106
Citations
1
Primary Topic
Atmospheric chemistry and aerosols
Type
article
Field-Weighted Citation Impact
0.38
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article

Illumination conditions of photocatalyst-containing mist on the degradation of organic compounds

Guoqing Guan, Yasuki Kansha, Shoma Kato, Yuka Sakai
1 citations
Chemical Engineering and Processing - Process Intensification
Atmospheric chemistry and aerosols
0.38
article

Illumination conditions of photocatalyst-containing mist on the degradation of organic compounds

Guoqing Guan, Yasuki Kansha, Shoma Kato, Yuka Sakai
article en
1 citations

Abstract

• The illumination conditions of photocatalyst-containing mist were studied. • UV light, ultrasound, and mist were applied to a mixture of TiO 2 and phenol. • Higher light intensities provided to the mist improved phenol degradation. • Excess TiO 2 prevented mist generation and utilization. • Findings inform the design of reactors that use photocatalysts and mist. Photocatalysis is a promising method for treating wastewater containing toxic organic pollutants. To improve the degradation of those pollutants, the utilization of mist that contains photocatalysts has been considered. In this study, the light illumination conditions of the mist that affect photocatalytic degradation were investigated to provide insight into the design of reactors that utilize photocatalyst-containing mist. In the reactor, UV light, ultrasound (US), and US-generated mist were applied to a mixture containing the TiO 2 photocatalyst and phenol as the model organic pollutant. The results indicated that higher UV intensities and TiO 2 dosages affected the illumination conditions to improve the degradation of phenol. However, at higher TiO 2 dosages, mist was not generated, so its enhanced illumination was not utilized in the degradation reactions. The analysis of the reaction kinetics suggested the enhancement of the illumination condition by the mist. These findings provide insight into the design of the reactor that utilizes photocatalyst-containing mist to improve the irradiation conditions and promote photocatalytic reactions.

Chemical Engineering and Processing - Process IntensificationVol. 208
Hirosaki University (JP), The University of Tokyo (JP)
Openalex Percentile: Top 38%
Atmospheric chemistry and aerosols
0.38
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Illumination conditions of photocatalyst-containing mist on the degradation of organic compounds — Guoqing Guan, Yasuki Kansha, et al. · Chemical Engineering and Processing - Process Intensification (2024) | TGRS Research Map | TGRS