Unveiling the Nontrivial Electronic Structures and Fermi Topology of High-Temperature Kagome Ferrimagnet HoMn<sub>6</sub>Sn<sub>6</sub>

High-temperature (HT) kagome magnets provide important platforms to explore nontrivial topological physics and promising potentials for spintronic applications, due to the complicated interactions among their electrons, lattices, and magnetism. Herein, the nontrivial electronic properties of a HT layered kagome-magnet, HoMn<sub>6</sub>Sn<sub>6</sub>, are systematically resolved by quantum oscillation measurements and density functional theory (DFT) calculations. The prominent Shubnikov-de Haas (SdH) oscillations under pulsed high magnetic fields reveal a high quantum mobility of 0.37 m<sup>2</sup>·V<sup>-1</sup>·s<sup>-1</sup> for this HT ferrimagnet. The observed multiple-frequency quantum oscillations exhibit various angular dependences, consistent with DFT calculations which suggest a complex Fermi topology of three three-dimensional hole pockets and two electron pockets. The observed π shift of the Berry phase for quantum oscillations unveils nontrivial topological properties in HoMn<sub>6</sub>Sn<sub>6</sub>, further confirmed by DFT calculated Dirac fermions and large anomalous Hall conductivity. Our findings establish HoMn<sub>6</sub>Sn<sub>6</sub> as an HT magnetic candidate for topological magnetoelectronics or spin quantum applications.

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Publication Details

Journal
Nano Letters
Published
2024-11-29
DOI
https://doi.org/10.1021/acs.nanolett.4c04411
Citations
1
Primary Topic
Topological Materials and Phenomena
Type
article
Field-Weighted Citation Impact
0.34

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article

Unveiling the Nontrivial Electronic Structures and Fermi Topology of High-Temperature Kagome Ferrimagnet HoMn6Sn6

Yusheng Hou, Detong Wu, Bing Shen, Meng Wang et al.
1 citations
Nano Letters
Topological Materials and Phenomena
0.34
article

Unveiling the Nontrivial Electronic Structures and Fermi Topology of High-Temperature Kagome Ferrimagnet HoMn6Sn6

Yusheng Hou, Detong Wu, Bing Shen, Meng Wang, Bin Wang, Huakun Zuo, Xiang-Fan Huang
article en
1 citations

Abstract

High-temperature (HT) kagome magnets provide important platforms to explore nontrivial topological physics and promising potentials for spintronic applications, due to the complicated interactions among their electrons, lattices, and magnetism. Herein, the nontrivial electronic properties of a HT layered kagome-magnet, HoMn<sub>6</sub>Sn<sub>6</sub>, are systematically resolved by quantum oscillation measurements and density functional theory (DFT) calculations. The prominent Shubnikov-de Haas (SdH) oscillations under pulsed high magnetic fields reveal a high quantum mobility of 0.37 m<sup>2</sup>·V<sup>-1</sup>·s<sup>-1</sup> for this HT ferrimagnet. The observed multiple-frequency quantum oscillations exhibit various angular dependences, consistent with DFT calculations which suggest a complex Fermi topology of three three-dimensional hole pockets and two electron pockets. The observed π shift of the Berry phase for quantum oscillations unveils nontrivial topological properties in HoMn<sub>6</sub>Sn<sub>6</sub>, further confirmed by DFT calculated Dirac fermions and large anomalous Hall conductivity. Our findings establish HoMn<sub>6</sub>Sn<sub>6</sub> as an HT magnetic candidate for topological magnetoelectronics or spin quantum applications.

Nano LettersVol. 24(50)
Sun Yat-sen University (CN)
National Natural Science Foundation of China, National Key Research and Development Program of China
Openalex Percentile: Top 38%
Topological Materials and Phenomena
0.34
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