Million-Q free space meta-optical resonator at near-visible wavelengths

High-quality (Q)-factor optical resonators with extreme temporal coherence are of both technological and fundamental importance in optical metrology, continuous-wave lasing, and semiconductor quantum optics. Despite extensive efforts in designing high-Q resonators across different spectral regimes, the experimental realization of very large Q-factors at visible wavelengths remains challenging due to the small feature size that is sensitive to fabrication imperfections, and thus is typically implemented in integrated photonics. In the pursuit of free-space optics with the benefits of large space-bandwidth product and massive parallel operations, here we design and fabricate a near-visible-wavelength etch-free metasurface with minimized fabrication defects and experimentally demonstrate a million-scale ultrahigh-Q resonance. A new laser-scanning momentum-space-resolved spectroscopy technique with extremely high spectral and angular resolution is developed to characterize the record-high Q-factor as well as the dispersion of the million-Q resonance in free space. By integrating monolayer WSe<sub>2</sub> into our ultrahigh-Q meta-resonator, we further demonstrate laser-like highly unidirectional and narrow-linewidth exciton emission, albeit without any operating power density threshold. Under continuous-wave laser pumping, we observe pump-power-dependent linewidth narrowing at room temperature, indicating the potential of our meta-optics platform in controlling coherent quantum light-sources. Our result also holds great promise for applications like optical sensing, spectral filtering, and few-photon nonlinear optics.

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Publication Details

Journal
Nature Communications
Published
2024-11-28
DOI
https://doi.org/10.1038/s41467-024-54775-0
Citations
20
Primary Topic
Photonic and Optical Devices
Type
article
Field-Weighted Citation Impact
4.17

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article

Million-Q free space meta-optical resonator at near-visible wavelengths

Andrea Alù, Vinod M. Menon, Arka Majumdar, Jie Fang et al.
20 citations
Nature Communications
Photonic and Optical Devices
4.17
article

Million-Q free space meta-optical resonator at near-visible wavelengths

Andrea Alù, Vinod M. Menon, Arka Majumdar, Jie Fang, Arnab Manna, David Sharp, Sander A. Mann, Andrew Tang, Enrico M. Renzi, Yuebing Zheng, Kan Yao, Christopher Munley, Abhinav Kala, Sinabu Pumulo, Hannah Rarick, Rui Chen
article en
20 citations

Abstract

High-quality (Q)-factor optical resonators with extreme temporal coherence are of both technological and fundamental importance in optical metrology, continuous-wave lasing, and semiconductor quantum optics. Despite extensive efforts in designing high-Q resonators across different spectral regimes, the experimental realization of very large Q-factors at visible wavelengths remains challenging due to the small feature size that is sensitive to fabrication imperfections, and thus is typically implemented in integrated photonics. In the pursuit of free-space optics with the benefits of large space-bandwidth product and massive parallel operations, here we design and fabricate a near-visible-wavelength etch-free metasurface with minimized fabrication defects and experimentally demonstrate a million-scale ultrahigh-Q resonance. A new laser-scanning momentum-space-resolved spectroscopy technique with extremely high spectral and angular resolution is developed to characterize the record-high Q-factor as well as the dispersion of the million-Q resonance in free space. By integrating monolayer WSe<sub>2</sub> into our ultrahigh-Q meta-resonator, we further demonstrate laser-like highly unidirectional and narrow-linewidth exciton emission, albeit without any operating power density threshold. Under continuous-wave laser pumping, we observe pump-power-dependent linewidth narrowing at room temperature, indicating the potential of our meta-optics platform in controlling coherent quantum light-sources. Our result also holds great promise for applications like optical sensing, spectral filtering, and few-photon nonlinear optics.

Nature CommunicationsVol. 15(1)
The Graduate Center, CUNY (US), City College of New York (US), City University of New York (US), University of Washington (US), CUNY Advanced Science Research Center (US), University of Washington Applied Physics Laboratory (US), Walker (United States) (US), The University of Texas at Austin (US)
National Science Foundation, University of Washington, National Institutes of Health, National Institute of General Medical Sciences, Division of Materials Research, Air Force Office of Scientific Research
Affordable and clean energy
Openalex Percentile: Top 5%
Photonic and Optical Devices
4.17
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