Theory of magnetotrion-polaritons in transition metal dichalcogenide monolayers

Magnetic field is a powerful tool for the manipulation of material’s electronic and optical properties. In the domain of transition metal dichalcogenide monolayers, it allows one to unveil the spin, valley, and orbital properties of many-body excitonic complexes. Here we study theoretically the impact of normal-to-plane magnetic field on trions and trion-polaritons. We demonstrate that spin and orbital effects of a magnetic field give comparable contributions to the trion energies. Moreover, as magnetic field redistributes the free electron gas between two valleys in the conductance band, the trion-photon coupling becomes polarization and valley dependent. This results in an effective giant Zeeman splitting of trion-polaritons, in-line with the recent experimental observations.

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Publication Details

Journal
npj 2D Materials and Applications
Published
2024-11-27
DOI
https://doi.org/10.1038/s41699-024-00517-1
Citations
2
Primary Topic
2D Materials and Applications
Type
article
Field-Weighted Citation Impact
0.23

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article

Theory of magnetotrion-polaritons in transition metal dichalcogenide monolayers

Zaur Alisultanov, I. A. Aleksandrov, K. Varga, V. Shahnazaryan et al.
2 citations
npj 2D Materials and Applications
2D Materials and Applications
0.23
article

Theory of magnetotrion-polaritons in transition metal dichalcogenide monolayers

Zaur Alisultanov, I. A. Aleksandrov, K. Varga, V. Shahnazaryan, I. A. Shelykh, A. Kudlis
article en
2 citations

Abstract

Magnetic field is a powerful tool for the manipulation of material’s electronic and optical properties. In the domain of transition metal dichalcogenide monolayers, it allows one to unveil the spin, valley, and orbital properties of many-body excitonic complexes. Here we study theoretically the impact of normal-to-plane magnetic field on trions and trion-polaritons. We demonstrate that spin and orbital effects of a magnetic field give comparable contributions to the trion energies. Moreover, as magnetic field redistributes the free electron gas between two valleys in the conductance band, the trion-photon coupling becomes polarization and valley dependent. This results in an effective giant Zeeman splitting of trion-polaritons, in-line with the recent experimental observations.

npj 2D Materials and ApplicationsVol. 8(1)
University of Iceland (IS), St Petersburg University (RU), ITMO University (RU), Vanderbilt University (US), Dagestan Scientific Center of the Russian Academy of Sciences (RU), Ioffe Institute (RU)
National Science Foundation, Rannís, Ministry of Science and Higher Education of the Russian Federation, Division of Materials Research
Openalex Percentile: Top 50%
2D Materials and Applications
0.23
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Theory of magnetotrion-polaritons in transition metal dichalcogenide monolayers — Zaur Alisultanov, I. A. Aleksandrov, et al. · npj 2D Materials and Applications (2024) | TGRS Research Map | TGRS