Theory of Gas Purification by Liquid Absorber in Small Rotating Channels with Application to the Patented Rotational Absorber Device

A new design for absorbing vapour-phase impurities from gases is presented. It consists of small channels packed in a rotating vertical cylinder. Gas flows through the channels adjacent to a thin film of absorber liquid. The liquid film is pressed to the radially outward side of each channel by the centrifugal force and flows downwards by gravity. Formulae are presented which describe the concentration distributions of gaseous impurities subject to absorption in gas and liquid. Results include expressions for laminar and turbulent diffusion coefficients to be used in mass balance equations. The role of rotation is quantified including the effect on wavy motion and enhanced diffusion in the liquid layer. Application in design is indicated for the case of separation of the greenhouse gas CO2 from flue gases of fossil fuel combustion processes. At other equal dimensions, the height of the Rotational Absorber Device is calculated to be 25 times shorter than the enormous heights of conventional tray and packed columns.

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Publication Details

Journal
Separations
Published
2024-11-26
DOI
https://doi.org/10.3390/separations11120338
Primary Topic
Cyclone Separators and Fluid Dynamics
Type
article
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article

Theory of Gas Purification by Liquid Absorber in Small Rotating Channels with Application to the Patented Rotational Absorber Device

J.J.H. Brouwers
Separations
Cyclone Separators and Fluid Dynamics
article

Theory of Gas Purification by Liquid Absorber in Small Rotating Channels with Application to the Patented Rotational Absorber Device

J.J.H. Brouwers
article en

Abstract

A new design for absorbing vapour-phase impurities from gases is presented. It consists of small channels packed in a rotating vertical cylinder. Gas flows through the channels adjacent to a thin film of absorber liquid. The liquid film is pressed to the radially outward side of each channel by the centrifugal force and flows downwards by gravity. Formulae are presented which describe the concentration distributions of gaseous impurities subject to absorption in gas and liquid. Results include expressions for laminar and turbulent diffusion coefficients to be used in mass balance equations. The role of rotation is quantified including the effect on wavy motion and enhanced diffusion in the liquid layer. Application in design is indicated for the case of separation of the greenhouse gas CO2 from flue gases of fossil fuel combustion processes. At other equal dimensions, the height of the Rotational Absorber Device is calculated to be 25 times shorter than the enormous heights of conventional tray and packed columns.

SeparationsVol. 11(12)
Openalex Percentile: Top 77%
Cyclone Separators and Fluid Dynamics
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