Electrically Generated Exciton Polaritons with Spin On‐Demand

Generation and manipulation of exciton polaritons with controllable spin could deeply impact spintronic applications, quantum simulations, and quantum information processing, but is inherently challenging due to the charge neutrality of the polariton and the device complexity it requires. Here, electrical generation of spin-polarized exciton polaritons in a monolithic dielectric perovskite metasurface embedded in a light-emitting transistor is demonstrated. A finely tailored interplay of in- and out-of-plane symmetry breaking of the metasurface allows to lift the spin degeneracy through the polaritonic Rashba effect, yielding high spin purity with normalized Stokes parameter of S<sub>3</sub> ≈ 0.8. Leveraging on spin-momentum locking, the unique metatransistor device architecture enables electrical control of spin and directionality of the polaritonic emission. Here, the development of compact and tunable spintronic devices is advanced and an important step toward the realization of electrically pumped inversionless spin-lasers is represented.

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Publication Details

Journal
Advanced Materials
Published
2024-11-26
DOI
https://doi.org/10.1002/adma.202412952
Citations
5
Primary Topic
Strong Light-Matter Interactions
Type
article
Field-Weighted Citation Impact
1.69

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article

Electrically Generated Exciton Polaritons with Spin On‐Demand

Cesare Soci, Giorgio Adamo, Son Tung Ha, Jingyi Tian et al.
5 citations
Advanced Materials
Strong Light-Matter Interactions
1.69
article

Electrically Generated Exciton Polaritons with Spin On‐Demand

Cesare Soci, Giorgio Adamo, Son Tung Ha, Jingyi Tian, Yutao Wang
article en
5 citations

Abstract

Generation and manipulation of exciton polaritons with controllable spin could deeply impact spintronic applications, quantum simulations, and quantum information processing, but is inherently challenging due to the charge neutrality of the polariton and the device complexity it requires. Here, electrical generation of spin-polarized exciton polaritons in a monolithic dielectric perovskite metasurface embedded in a light-emitting transistor is demonstrated. A finely tailored interplay of in- and out-of-plane symmetry breaking of the metasurface allows to lift the spin degeneracy through the polaritonic Rashba effect, yielding high spin purity with normalized Stokes parameter of S<sub>3</sub> ≈ 0.8. Leveraging on spin-momentum locking, the unique metatransistor device architecture enables electrical control of spin and directionality of the polaritonic emission. Here, the development of compact and tunable spintronic devices is advanced and an important step toward the realization of electrically pumped inversionless spin-lasers is represented.

Advanced MaterialsVol. 37(8)
Agency for Science, Technology and Research (SG), Nanyang Technological University (SG), Westlake University (CN), Université Bourgogne Franche-Comté (FR), Institute of Materials Research and Engineering (SG)
Agency for Science, Technology and Research, Ministry of Education - Singapore
Affordable and clean energy
Openalex Percentile: Top 16%
Strong Light-Matter Interactions
1.69
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