Etchless Dion–Jacobson-Phase Perovskite Surface-Emitting Circular Bragg Lasers with an Ultrahigh <i>Q</i> Factor
Metal halide perovskites are an excellent direct-bandgap semiconductor material that can possess high optical gain for laser and amplifier applications. Engineering light–matter interactions in perovskites by using a circular Bragg cavity holds great promise for high-performance on-chip photonic sources. Here, we report our development of an etchless fabrication method for perovskite active photonics with an experimental demonstration of circular Bragg lasers in quasi-2D Dion–Jacobson-phase perovskites. The demonstrated perovskite lasers exhibit excellent performance including a low lasing threshold of 8 μJ/cm2 and a record-high quality factor of ∼1.2 × 104. These laser devices have excellent stability due to the adoption of the Dion–Jacobson-phase perovskite and material-compatible fabrication processing. This work opens a new avenue to large-area, single-mode surface-emitting perovskite lasers and also provides a new platform for perovskite integrated photonics.
Authors
- Xue-Zhou Wang (ORCID: https://orcid.org/0000-0003-0731-7257)
- Xiankai Sun (ORCID: https://orcid.org/0000-0002-9137-0298)
- Ziyao Feng (ORCID: https://orcid.org/0000-0003-0268-9211)
- Li Zeng (ORCID: https://orcid.org/0000-0001-6390-0370)
- Ni Zhao (ORCID: https://orcid.org/0000-0002-1536-8516)
- Long Jin (ORCID: https://orcid.org/0009-0006-5148-5089)
Institutions
- Chinese University of Hong Kong (HK)
Publication Details
- Journal
- ACS Photonics
- Published
- 2024-11-25
- DOI
- https://doi.org/10.1021/acsphotonics.4c00880
- Citations
- 4
- Primary Topic
- Perovskite Materials and Applications
- Type
- article
- Field-Weighted Citation Impact
- 0.83
Funders
- Research Grants Council, University Grants Committee
- Chinese University of Hong Kong