Ultrafast optical induction of magnetic order at a quantum critical point

Time-resolved ultrafast spectroscopy has emerged as a promising tool to dynamically induce and manipulate non-trivial electronic states of matter out-of-equilibrium. Here we theoretically investigate light pulse driven dynamics in a Kondo lattice system close to quantum criticality. Based on a time-dependent auxiliary fermion mean-field calculation we show that light can dehybridize the local Kondo screening and induce oscillating magnetic order out of a previously paramagnetic state. Depending on the laser pulse field amplitude and frequency the Kondo singlet can be completely deconfined, inducing a dynamic Lifshitz transition that changes the Fermi surface topology. These phenomena can be identified in harmonic generation and time-resolved angle-resolved photoemission spectroscopy spectra. Our results shed new light on non-equilibrium states in heavy fermion systems.

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Publication Details

Journal
Journal of Physics Condensed Matter
Published
2024-11-22
DOI
https://doi.org/10.1088/1361-648x/ad9659
Citations
2
Primary Topic
Quantum and electron transport phenomena
Type
article
Field-Weighted Citation Impact
0.68

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article

Ultrafast optical induction of magnetic order at a quantum critical point

Benedikt Fauseweh, Jian‐Xin Zhu
2 citations
Journal of Physics Condensed Matter
Quantum and electron transport phenomena
0.68
article

Ultrafast optical induction of magnetic order at a quantum critical point

Benedikt Fauseweh, Jian‐Xin Zhu
article en
2 citations

Abstract

Time-resolved ultrafast spectroscopy has emerged as a promising tool to dynamically induce and manipulate non-trivial electronic states of matter out-of-equilibrium. Here we theoretically investigate light pulse driven dynamics in a Kondo lattice system close to quantum criticality. Based on a time-dependent auxiliary fermion mean-field calculation we show that light can dehybridize the local Kondo screening and induce oscillating magnetic order out of a previously paramagnetic state. Depending on the laser pulse field amplitude and frequency the Kondo singlet can be completely deconfined, inducing a dynamic Lifshitz transition that changes the Fermi surface topology. These phenomena can be identified in harmonic generation and time-resolved angle-resolved photoemission spectroscopy spectra. Our results shed new light on non-equilibrium states in heavy fermion systems.

Journal of Physics Condensed MatterVol. 37(7)
Los Alamos National Laboratory (US), TU Dortmund University (DE), Center for Integrated Nanotechnologies (US)
Los Alamos National Laboratory
Affordable and clean energy
Openalex Percentile: Top 30%
Quantum and electron transport phenomena
0.68
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