[111]-strained spin ice: Localization of thermodynamically deconfined monopoles

We study classical spin ice under uniaxial strain along the [111] crystallographic axis. Remarkably, such strain preserves the extensive ice degeneracy and the corresponding classical Coulomb phase. The emergent monopole excitations remain thermodynamically deconfined exactly as in the isotropic case. However, their motion under local heat bath dynamics depends qualitatively on the sign of the strain. In the low-temperature limit for negative strain, the monopoles diffuse, while for positive strain, they localize. Introducing additional ring exchange dynamics into the ice background transforms the localized monopoles into subdimensional excitations whose motion is restricted to diffusion in the (111)-plane. The phenomena we identify are experimentally accessible in rare-earth pyrochlores under uniaxial stress as well as in tripod kagome materials. The diffusive versus localized nature of the monopoles manifests in characteristic magnetic noise spectra, which we compute.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2024-11-21
DOI
https://doi.org/10.1103/physrevb.110.184421
Citations
5
Primary Topic
Advanced Condensed Matter Physics
Type
article
Field-Weighted Citation Impact
1.55

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article

[111]-strained spin ice: Localization of thermodynamically deconfined monopoles

Chris R. Laumann, Robin Schäfer, Jonathan N. Hallén, Zhongling Lu
5 citations
Physical review. B./Physical review. B
Advanced Condensed Matter Physics
1.55
article

[111]-strained spin ice: Localization of thermodynamically deconfined monopoles

Chris R. Laumann, Robin Schäfer, Jonathan N. Hallén, Zhongling Lu
article en
5 citations

Abstract

We study classical spin ice under uniaxial strain along the [111] crystallographic axis. Remarkably, such strain preserves the extensive ice degeneracy and the corresponding classical Coulomb phase. The emergent monopole excitations remain thermodynamically deconfined exactly as in the isotropic case. However, their motion under local heat bath dynamics depends qualitatively on the sign of the strain. In the low-temperature limit for negative strain, the monopoles diffuse, while for positive strain, they localize. Introducing additional ring exchange dynamics into the ice background transforms the localized monopoles into subdimensional excitations whose motion is restricted to diffusion in the (111)-plane. The phenomena we identify are experimentally accessible in rare-earth pyrochlores under uniaxial stress as well as in tripod kagome materials. The diffusive versus localized nature of the monopoles manifests in characteristic magnetic noise spectra, which we compute.

Physical review. B./Physical review. BVol. 110(18)
Boston University (US), Harvard University (US), Shanghai Jiao Tong University (CN), Harvard University Press (US), Max Planck Institute for the Physics of Complex Systems (DE)
Deutsche Forschungsgemeinschaft, Air Force Office of Scientific Research
Openalex Percentile: Top 17%
Advanced Condensed Matter Physics
1.55
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[111]-strained spin ice: Localization of thermodynamically deconfined monopoles — Chris R. Laumann, Robin Schäfer, et al. · Physical review. B./Physical review. B (2024) | TGRS Research Map | TGRS