Broad Range Tuning of InAs Quantum Dot Emission for Nanophotonic Devices in the Telecommunication Bands

InAs semiconductor quantum dots (QDs) emitting in the near-infrared are promising platforms for on-demand single-photon sources and spin-photon interfaces. However, the realization of quantum-photonic nanodevices emitting in the telecom windows with similar performance remains an open challenge. In particular, nanophotonic devices incorporating quantum light emitting diodes in the telecom C-band based on GaAs substrates are still lacking due to the relaxation of the lattice constant along the InGaAs graded layer which makes the implementation of electrically contacted devices challenging. Here, we report an optimized heterostructure design for QDs emitting in the telecom O- and C-bands grown by means of molecular beam epitaxy. The InAs QDs are embedded in mostly relaxed InGaAs matrices with fixed indium content grown on top of compositionally graded InGaAs buffers. Reciprocal space maps of the indium profiles and optical absorption spectra are used to optimize In<sub>0.22</sub>Ga<sub>0.78</sub>As and In<sub>0.30</sub>Ga<sub>0.70</sub>As matrices, accounting for the chosen indium grading profile. This approach results in a tunable QD photoluminescence (PL) emission from 1200 up to 1600 nm. Power and polarization dependent micro-PL measurements performed at 4 K reveal exciton-biexciton complexes from quantum dots emitting in the telecom O- and C-bands. The presented study establishes a flexible platform that can be an essential component for advanced photonic devices based on InAs/GaAs that serve as building blocks for future quantum networks.

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Publication Details

Journal
ACS Applied Nano Materials
Published
2024-11-20
DOI
https://doi.org/10.1021/acsanm.4c04810
Citations
7
Primary Topic
Semiconductor Quantum Structures and Devices
Type
article
Field-Weighted Citation Impact
2.36

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article

Broad Range Tuning of InAs Quantum Dot Emission for Nanophotonic Devices in the Telecommunication Bands

Gregor Koblmüller, Jonathan J. Finley, Elise Sirotti, Beatrice Costa et al.
7 citations
ACS Applied Nano Materials
Semiconductor Quantum Structures and Devices
2.36
article

Broad Range Tuning of InAs Quantum Dot Emission for Nanophotonic Devices in the Telecommunication Bands

Gregor Koblmüller, Jonathan J. Finley, Elise Sirotti, Beatrice Costa, Bianca Scaparra, Pavel Avdienko, Hubert Riedl, Akhil Ajay, Björn Jonas, Ian D. Sharp, Eugenio Zallo, Kai Müller
article en
7 citations

Abstract

InAs semiconductor quantum dots (QDs) emitting in the near-infrared are promising platforms for on-demand single-photon sources and spin-photon interfaces. However, the realization of quantum-photonic nanodevices emitting in the telecom windows with similar performance remains an open challenge. In particular, nanophotonic devices incorporating quantum light emitting diodes in the telecom C-band based on GaAs substrates are still lacking due to the relaxation of the lattice constant along the InGaAs graded layer which makes the implementation of electrically contacted devices challenging. Here, we report an optimized heterostructure design for QDs emitting in the telecom O- and C-bands grown by means of molecular beam epitaxy. The InAs QDs are embedded in mostly relaxed InGaAs matrices with fixed indium content grown on top of compositionally graded InGaAs buffers. Reciprocal space maps of the indium profiles and optical absorption spectra are used to optimize In<sub>0.22</sub>Ga<sub>0.78</sub>As and In<sub>0.30</sub>Ga<sub>0.70</sub>As matrices, accounting for the chosen indium grading profile. This approach results in a tunable QD photoluminescence (PL) emission from 1200 up to 1600 nm. Power and polarization dependent micro-PL measurements performed at 4 K reveal exciton-biexciton complexes from quantum dots emitting in the telecom O- and C-bands. The presented study establishes a flexible platform that can be an essential component for advanced photonic devices based on InAs/GaAs that serve as building blocks for future quantum networks.

ACS Applied Nano MaterialsVol. 7(23)
Schott (Germany) (DE), Munich Center for Quantum Science and Technology (DE), Technical University of Munich (DE)
QuantIC, European Commission, Deutsche Forschungsgemeinschaft, Bundesministerium für Bildung und Forschung, Technische Universität München, Bayerische Staatsministerium für Wirtschaft, Landesentwicklung und Energie, Bayerisches Staatsministerium für Wissenschaft und Kunst, Munich Center for Quantum Science and Technology, H2020 European Research Council, H2020 Future and Emerging Technologies
Affordable and clean energy
Openalex Percentile: Top 11%
Semiconductor Quantum Structures and Devices
2.36
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