Designing rotational motion of charge densities on plasmonic nanostructures excited by circularly polarized light

Abstract Rotational motion of charges in plasmonic nanostructures plays an important role in transferring angular momentum between light and matter on the nanometer scale. Although sophisticated control of rotational charge motion has been achieved using spatially structured light, its extension to simultaneous excitation of the same charge motion in multiple nanostructures is not straightforward. In this study, we perform model calculations to show that spatially homogeneous circularly polarized (CP) light can excite rotational charge motions with a high degrees of freedom by exploiting the rotational symmetry of the plasmonic structure and that of the plasmon mode. Finite‐difference time‐domain simulations demonstrate selective excitation of rotational charge motion for both isolated nanoplates and periodic array structures, showing that complex charge rotations can be manipulated by plane CP waves in a wide range of plasmonic structures.