Laser-Induced Nanostructured Si and SiGe Layers for Enhanced Optical and Thermoelectric Performance

We investigate a method for fabricating layers that exhibit both high optical absorption and promising thermoelectric properties. Using plasma-enhanced chemical vapor deposition (PECVD), amorphous Si and Si<sub>72</sub>Ge<sub>28</sub> layers are deposited on glass substrates and subsequently processed via laser annealing to achieve nanostructured layers. Our results show that a single laser annealing pulse at 40 mJ yields the highest power factor, approximately 90 μW/m·K<sup>2</sup>. Additionally, we observe a maximum absorbance enhancement factor of 60 times in the spectral region near 880 nm for samples treated with a single pulse of 60 mJ compared to untreated samples. The effects of laser energy, the number of pulses, and material choice are further discussed.

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Publication Details

Journal
ACS Omega
Published
2024-11-20
DOI
https://doi.org/10.1021/acsomega.4c06006
Primary Topic
Advanced Thermoelectric Materials and Devices
Type
article
Field-Weighted Citation Impact
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article

Laser-Induced Nanostructured Si and SiGe Layers for Enhanced Optical and Thermoelectric Performance

Fabien Giovannelli, Eliane Bsaibess, Stavros Christopoulos, Ahmed Slimani et al.
ACS Omega
Advanced Thermoelectric Materials and Devices
article

Laser-Induced Nanostructured Si and SiGe Layers for Enhanced Optical and Thermoelectric Performance

Fabien Giovannelli, Eliane Bsaibess, Stavros Christopoulos, Ahmed Slimani, Joumana El-Rifai, Valerie Laux-Le Guyon
article en

Abstract

We investigate a method for fabricating layers that exhibit both high optical absorption and promising thermoelectric properties. Using plasma-enhanced chemical vapor deposition (PECVD), amorphous Si and Si<sub>72</sub>Ge<sub>28</sub> layers are deposited on glass substrates and subsequently processed via laser annealing to achieve nanostructured layers. Our results show that a single laser annealing pulse at 40 mJ yields the highest power factor, approximately 90 μW/m·K<sup>2</sup>. Additionally, we observe a maximum absorbance enhancement factor of 60 times in the spectral region near 880 nm for samples treated with a single pulse of 60 mJ compared to untreated samples. The effects of laser energy, the number of pulses, and material choice are further discussed.

ACS OmegaVol. 9(48)
Université de Tours (FR), Centre National de la Recherche Scientifique (FR), Services déconcentrés d'appui à la recherche Val de Loire (FR), Sorbonne University Abu Dhabi (AE), Institut National des Sciences Appliquées Centre Val de Loire (FR)
Affordable and clean energy
Openalex Percentile: Top 87%
Advanced Thermoelectric Materials and Devices
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