Observation of Linear Resistance at Low Temperatures in Hole-Doped Degenerate Spin-Valley Semiconductors

Linear resistivity-temperature (<i>R</i>-<i>T</i>) at low temperatures, referred to as strange metal (SM), is an unusual characteristic observed in strongly correlated systems. SM is often mingled with superconductivity and magnetism in various materials. Here, we report a linear <i>R</i>-<i>T</i> relation in a hole-doped, degenerate spin-valley (SV) semiconductor, V<sub>0.25</sub>W<sub>0.75</sub>Se<sub>2</sub>, with hole pockets in the valence band. SM emerges over a wide temperature range (1.8-150 K) without any apparent superconductivity down to 110 mK. This SM behavior is suppressed at low temperatures below 20 K in the presence of a magnetic field. The ansatz <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mi>R</mml:mi><mml:mrow><mml:mo>(</mml:mo><mml:mi>H</mml:mi><mml:mo>,</mml:mo><mml:mi>T</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mo>-</mml:mo><mml:mi>R</mml:mi><mml:mrow><mml:mo>(</mml:mo><mml:mn>0</mml:mn><mml:mo>,</mml:mo><mml:mn>0</mml:mn><mml:mo>)</mml:mo></mml:mrow><mml:mo>∝</mml:mo><mml:msqrt><mml:mrow><mml:msup><mml:mrow><mml:mrow><mml:mo>(</mml:mo><mml:mi>α</mml:mi><mml:msub><mml:mrow><mml:mi>k</mml:mi></mml:mrow><mml:mrow><mml:mi>B</mml:mi></mml:mrow></mml:msub><mml:mi>T</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msup><mml:mo>+</mml:mo><mml:msup><mml:mrow><mml:mrow><mml:mo>(</mml:mo><mml:mi>γ</mml:mi><mml:msub><mml:mrow><mml:mi>μ</mml:mi></mml:mrow><mml:mrow><mml:mi>B</mml:mi></mml:mrow></mml:msub><mml:msub><mml:mrow><mml:mi>μ</mml:mi></mml:mrow><mml:mrow><mml:mn>0</mml:mn></mml:mrow></mml:msub><mml:mi>H</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:msqrt></mml:math> yields the γ/α ratio of ∼4, larger than the previous reports. The observed SM over a wide temperature range is explained by a spin-orbit coupling (SOC)-mediated SV pair with strong correlation effects, analogous to a phonon-mediated Cooper pair in superconductivity. This finding opens possible routes for understanding strange metal behavior through the interplay of strong SOC and strong Coulomb interactions.

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Journal
Nano Letters
Published
2024-11-20
DOI
https://doi.org/10.1021/acs.nanolett.4c04247
Primary Topic
Magnetic and transport properties of perovskites and related materials
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article
Field-Weighted Citation Impact
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article

Observation of Linear Resistance at Low Temperatures in Hole-Doped Degenerate Spin-Valley Semiconductors

Tuan Dung Nguyen, Seon Je Kim, Dinh Loc Duong⧫, Mallesh Baithi et al.
Nano Letters
Magnetic and transport properties of perovskites and related materials
article

Observation of Linear Resistance at Low Temperatures in Hole-Doped Degenerate Spin-Valley Semiconductors

Tuan Dung Nguyen, Seon Je Kim, Dinh Loc Duong⧫, Mallesh Baithi, Young‐Min Kim, Young Hee Lee
article en

Abstract

Linear resistivity-temperature (<i>R</i>-<i>T</i>) at low temperatures, referred to as strange metal (SM), is an unusual characteristic observed in strongly correlated systems. SM is often mingled with superconductivity and magnetism in various materials. Here, we report a linear <i>R</i>-<i>T</i> relation in a hole-doped, degenerate spin-valley (SV) semiconductor, V<sub>0.25</sub>W<sub>0.75</sub>Se<sub>2</sub>, with hole pockets in the valence band. SM emerges over a wide temperature range (1.8-150 K) without any apparent superconductivity down to 110 mK. This SM behavior is suppressed at low temperatures below 20 K in the presence of a magnetic field. The ansatz <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mi>R</mml:mi><mml:mrow><mml:mo>(</mml:mo><mml:mi>H</mml:mi><mml:mo>,</mml:mo><mml:mi>T</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mo>-</mml:mo><mml:mi>R</mml:mi><mml:mrow><mml:mo>(</mml:mo><mml:mn>0</mml:mn><mml:mo>,</mml:mo><mml:mn>0</mml:mn><mml:mo>)</mml:mo></mml:mrow><mml:mo>∝</mml:mo><mml:msqrt><mml:mrow><mml:msup><mml:mrow><mml:mrow><mml:mo>(</mml:mo><mml:mi>α</mml:mi><mml:msub><mml:mrow><mml:mi>k</mml:mi></mml:mrow><mml:mrow><mml:mi>B</mml:mi></mml:mrow></mml:msub><mml:mi>T</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msup><mml:mo>+</mml:mo><mml:msup><mml:mrow><mml:mrow><mml:mo>(</mml:mo><mml:mi>γ</mml:mi><mml:msub><mml:mrow><mml:mi>μ</mml:mi></mml:mrow><mml:mrow><mml:mi>B</mml:mi></mml:mrow></mml:msub><mml:msub><mml:mrow><mml:mi>μ</mml:mi></mml:mrow><mml:mrow><mml:mn>0</mml:mn></mml:mrow></mml:msub><mml:mi>H</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:msqrt></mml:math> yields the γ/α ratio of ∼4, larger than the previous reports. The observed SM over a wide temperature range is explained by a spin-orbit coupling (SOC)-mediated SV pair with strong correlation effects, analogous to a phonon-mediated Cooper pair in superconductivity. This finding opens possible routes for understanding strange metal behavior through the interplay of strong SOC and strong Coulomb interactions.

Nano LettersVol. 24(48)
Institute for Basic Science (KR), Hubei University of Technology (CN), University of Maine (US), Sungkyunkwan University (KR)
National Research Foundation of Korea, Institute for Basic Science
Openalex Percentile: Top 88%
Magnetic and transport properties of perovskites and related materials
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