Time-resolved magneto-optical effects in the altermagnet candidate MnTe

α -MnTe is an antiferromagnetic semiconductor with above room temperature TN = 310 K, which is promising for spintronic applications. Recently, it was reported to be an altermagnet, containing bands with momentum-dependent spin splitting; time-resolved experimental probes of MnTe are, therefore, important both for understanding novel magnetic properties and potential device applications. We investigate ultrafast spin dynamics in epitaxial MnTe(001)/InP(111) thin films using pump-probe magneto-optical measurements in the Kerr configuration. At room temperature, we observe an oscillation mode at 55 GHz that does not appear at zero magnetic field. Combining field and polarization dependence, we identify this mode as a magnon, likely originating from inverse stimulated Raman scattering. Magnetic field-dependent oscillations persist up to at least 335 K, which could reflect coupling to known short-range magnetic order in MnTe above TN. Additionally, we observe two optical phonons at 3.6 and 4.2 THz, which broaden and redshift with increasing temperature.

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Publication Details

Journal
Applied Physics Letters
Published
2024-11-18
DOI
https://doi.org/10.1063/5.0244878
Citations
27
Primary Topic
Magnetic properties of thin films
Type
article
Field-Weighted Citation Impact
9.11

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article

Time-resolved magneto-optical effects in the altermagnet candidate MnTe

J. Steven Dodge, Isaiah Gray, Matthew Brahlek, Michael Chilcote et al.
27 citations
Applied Physics Letters
Magnetic properties of thin films
9.11
article

Time-resolved magneto-optical effects in the altermagnet candidate MnTe

J. Steven Dodge, Isaiah Gray, Matthew Brahlek, Michael Chilcote, Liang Wu, Qinwen Deng, Qi Tian
article en
27 citations

Abstract

α -MnTe is an antiferromagnetic semiconductor with above room temperature TN = 310 K, which is promising for spintronic applications. Recently, it was reported to be an altermagnet, containing bands with momentum-dependent spin splitting; time-resolved experimental probes of MnTe are, therefore, important both for understanding novel magnetic properties and potential device applications. We investigate ultrafast spin dynamics in epitaxial MnTe(001)/InP(111) thin films using pump-probe magneto-optical measurements in the Kerr configuration. At room temperature, we observe an oscillation mode at 55 GHz that does not appear at zero magnetic field. Combining field and polarization dependence, we identify this mode as a magnon, likely originating from inverse stimulated Raman scattering. Magnetic field-dependent oscillations persist up to at least 335 K, which could reflect coupling to known short-range magnetic order in MnTe above TN. Additionally, we observe two optical phonons at 3.6 and 4.2 THz, which broaden and redshift with increasing temperature.

Applied Physics LettersVol. 125(21)
Oak Ridge National Laboratory (US), Simon Fraser University (CA), University of Pennsylvania (US)
Office of Naval Research, Basic Energy Sciences, Air Force Office of Scientific Research, Army Research Office
Affordable and clean energy
Openalex Percentile: Top 1%
Magnetic properties of thin films
9.11
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