Pt-Nanoparticle-Loaded Porous SnO<sub>2</sub> for Optimizing H<sub>2</sub>S-Sensing Performance at Room Temperature
Achieving the real-time detection of hydrogen sulfide (H2S) based on metal oxide semiconductor (MOS) gas sensors is of great significance for rapid disease diagnosis. However, the high-power consumption and poor selectivity severely limit its practice application. In this study, a platinum nanoparticle (Pt NPs)-loaded porous metal–organic framework (MOF)-derived SnO2 material was successfully synthesized to optimize the H2S-sensing performance at room temperature. The optimized Pt-loaded porous SnO2-based gas sensor exhibited remarkably high sensitivity (712–10 ppm), fast response (21 s), good selectivity, and extremely low detection limit for H2S (10 ppb) at room temperature. The in-depth analysis demonstrated that the porous structure of Sn-MOF can provide adequate active reaction sites for gas molecules. Moreover, the uniform distribution of surface-loaded Pt NPs can initiate electron and chemical sensitization effects, thereby improving the sensing performance. The successful application of Pt NPs provides a novel approach to improve the room-temperature (RT) sensing performance of metal-oxide-semiconductor-based gas sensors.
Authors
- Xiaoxiong Hou
- Zihuan Tang
- Xiaotong Gao
- Zhuangzhuang Ma (ORCID: https://orcid.org/0000-0002-7534-5826)
- Lichao Jia (ORCID: https://orcid.org/0000-0003-3291-3632)
- Peijin Zou
Institutions
- Wuhan University of Science and Technology (CN)
- Shaanxi Normal University (CN)
Publication Details
- Journal
- ACS ES&T Engineering
- Published
- 2024-11-19
- DOI
- https://doi.org/10.1021/acsestengg.4c00522
- Citations
- 6
- Primary Topic
- Gas Sensing Nanomaterials and Sensors
- Type
- article
- Field-Weighted Citation Impact
- 1.25
Funders
- State Key Laboratory of Solidification Processing