Pt-Nanoparticle-Loaded Porous SnO<sub>2</sub> for Optimizing H<sub>2</sub>S-Sensing Performance at Room Temperature

Achieving the real-time detection of hydrogen sulfide (H2S) based on metal oxide semiconductor (MOS) gas sensors is of great significance for rapid disease diagnosis. However, the high-power consumption and poor selectivity severely limit its practice application. In this study, a platinum nanoparticle (Pt NPs)-loaded porous metal–organic framework (MOF)-derived SnO2 material was successfully synthesized to optimize the H2S-sensing performance at room temperature. The optimized Pt-loaded porous SnO2-based gas sensor exhibited remarkably high sensitivity (712–10 ppm), fast response (21 s), good selectivity, and extremely low detection limit for H2S (10 ppb) at room temperature. The in-depth analysis demonstrated that the porous structure of Sn-MOF can provide adequate active reaction sites for gas molecules. Moreover, the uniform distribution of surface-loaded Pt NPs can initiate electron and chemical sensitization effects, thereby improving the sensing performance. The successful application of Pt NPs provides a novel approach to improve the room-temperature (RT) sensing performance of metal-oxide-semiconductor-based gas sensors.

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Publication Details

Journal
ACS ES&T Engineering
Published
2024-11-19
DOI
https://doi.org/10.1021/acsestengg.4c00522
Citations
6
Primary Topic
Gas Sensing Nanomaterials and Sensors
Type
article
Field-Weighted Citation Impact
1.25

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article

Pt-Nanoparticle-Loaded Porous SnO2 for Optimizing H2S-Sensing Performance at Room Temperature

Xiaoxiong Hou, Zihuan Tang, Xiaotong Gao, Zhuangzhuang Ma et al.
6 citations
ACS ES&T Engineering
Gas Sensing Nanomaterials and Sensors
1.25
article

Pt-Nanoparticle-Loaded Porous SnO2 for Optimizing H2S-Sensing Performance at Room Temperature

Xiaoxiong Hou, Zihuan Tang, Xiaotong Gao, Zhuangzhuang Ma, Lichao Jia, Peijin Zou
article en
6 citations

Abstract

Achieving the real-time detection of hydrogen sulfide (H2S) based on metal oxide semiconductor (MOS) gas sensors is of great significance for rapid disease diagnosis. However, the high-power consumption and poor selectivity severely limit its practice application. In this study, a platinum nanoparticle (Pt NPs)-loaded porous metal–organic framework (MOF)-derived SnO2 material was successfully synthesized to optimize the H2S-sensing performance at room temperature. The optimized Pt-loaded porous SnO2-based gas sensor exhibited remarkably high sensitivity (712–10 ppm), fast response (21 s), good selectivity, and extremely low detection limit for H2S (10 ppb) at room temperature. The in-depth analysis demonstrated that the porous structure of Sn-MOF can provide adequate active reaction sites for gas molecules. Moreover, the uniform distribution of surface-loaded Pt NPs can initiate electron and chemical sensitization effects, thereby improving the sensing performance. The successful application of Pt NPs provides a novel approach to improve the room-temperature (RT) sensing performance of metal-oxide-semiconductor-based gas sensors.

ACS ES&T EngineeringVol. 5(1)
Wuhan University of Science and Technology (CN), Shaanxi Normal University (CN)
State Key Laboratory of Solidification Processing
Affordable and clean energy
Openalex Percentile: Top 20%
Gas Sensing Nanomaterials and Sensors
1.25
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Pt-Nanoparticle-Loaded Porous SnO<sub>2</sub> for Optimizing H<sub>2</sub>S-Sensing Performance at Room Temperature — Xiaoxiong Hou, Zihuan Tang, et al. · ACS ES&T Engineering (2024) | TGRS Research Map | TGRS