Fast-Response, Broadband Si-Based Photothermoelectric Photodetector Based on RF-Sputtering PbTe Film
Mid- and long-wave infrared photodetection is highly desired for various modern optoelectronic devices, but Si-based broadband photodetectors operating at room temperature remain challenging and are being extensively sought. In this paper, a Si-based photodetector with a broadband and fast photoresponse based on the photothermoelectric (PTE) effect of lead telluride (PbTe) film is demonstrated. Large-area, high-crystallinity PbTe film grown by a low-temperature, CMOS-compatible RF magnetron sputtering method is first reported for photodetection. The PbTe PTE photodetector surpasses the energy band gap limitation, operating even at wavelengths exceeding 10 μm. A rapid response time of less than 1 ms is obtained at 1310 nm, which is superior to those of most other reported PTE detectors. Furthermore, the development of a 5 × 5 array device shows a good photoresponse uniformity and demonstrates consistent mid-infrared imaging capabilities at room temperature. Excellent mechanical flexibility enables the integration of wearable optoelectronic devices. This pioneering research paves the way for significant advancements in Si-based broadband photodetector technologies, with potential applications in monolithic integrated detection and imaging systems that operate in visible- to long-wave infrared wavelengths at room temperature.
Authors
- Hang Yu (ORCID: https://orcid.org/0000-0003-2050-7346)
- Jiangchao Han (ORCID: https://orcid.org/0000-0002-5343-3091)
- Zhiming Wu (ORCID: https://orcid.org/0000-0003-3217-1376)
- Jun Gou (ORCID: https://orcid.org/0009-0004-8422-1421)
- Chunyu Li (ORCID: https://orcid.org/0000-0001-8124-2498)
- Jun Wang
- Lixin Liu (ORCID: https://orcid.org/0000-0001-6133-4977)
- He Yu (ORCID: https://orcid.org/0000-0002-4639-1321)
- Yadong Jiang
- Han Dou
- Xiutao Yang (ORCID: https://orcid.org/0009-0003-8506-4002)
Institutions
- University of Electronic Science and Technology of China (CN)
- Henan Tianguan Group (China) (CN)
- National Engineering Research Center of Electromagnetic Radiation Control Materials (CN)
Publication Details
- Journal
- ACS Photonics
- Published
- 2024-11-08
- DOI
- https://doi.org/10.1021/acsphotonics.4c01248
- Citations
- 9
- Primary Topic
- Advanced Thermoelectric Materials and Devices
- Type
- article
- Field-Weighted Citation Impact
- 1.05
Funders
- National Natural Science Foundation of China
- Aeronautical Science Foundation of China
- Natural Science Foundation of Sichuan Province