Fast-Response, Broadband Si-Based Photothermoelectric Photodetector Based on RF-Sputtering PbTe Film

Mid- and long-wave infrared photodetection is highly desired for various modern optoelectronic devices, but Si-based broadband photodetectors operating at room temperature remain challenging and are being extensively sought. In this paper, a Si-based photodetector with a broadband and fast photoresponse based on the photothermoelectric (PTE) effect of lead telluride (PbTe) film is demonstrated. Large-area, high-crystallinity PbTe film grown by a low-temperature, CMOS-compatible RF magnetron sputtering method is first reported for photodetection. The PbTe PTE photodetector surpasses the energy band gap limitation, operating even at wavelengths exceeding 10 μm. A rapid response time of less than 1 ms is obtained at 1310 nm, which is superior to those of most other reported PTE detectors. Furthermore, the development of a 5 × 5 array device shows a good photoresponse uniformity and demonstrates consistent mid-infrared imaging capabilities at room temperature. Excellent mechanical flexibility enables the integration of wearable optoelectronic devices. This pioneering research paves the way for significant advancements in Si-based broadband photodetector technologies, with potential applications in monolithic integrated detection and imaging systems that operate in visible- to long-wave infrared wavelengths at room temperature.

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Publication Details

Journal
ACS Photonics
Published
2024-11-08
DOI
https://doi.org/10.1021/acsphotonics.4c01248
Citations
9
Primary Topic
Advanced Thermoelectric Materials and Devices
Type
article
Field-Weighted Citation Impact
1.05

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article

Fast-Response, Broadband Si-Based Photothermoelectric Photodetector Based on RF-Sputtering PbTe Film

Hang Yu, Jiangchao Han, Zhiming Wu, Jun Gou et al.
9 citations
ACS Photonics
Advanced Thermoelectric Materials and Devices
1.05
article

Fast-Response, Broadband Si-Based Photothermoelectric Photodetector Based on RF-Sputtering PbTe Film

Hang Yu, Jiangchao Han, Zhiming Wu, Jun Gou, Chunyu Li, Jun Wang, Lixin Liu, He Yu, Yadong Jiang, Han Dou, Xiutao Yang
article en
9 citations

Abstract

Mid- and long-wave infrared photodetection is highly desired for various modern optoelectronic devices, but Si-based broadband photodetectors operating at room temperature remain challenging and are being extensively sought. In this paper, a Si-based photodetector with a broadband and fast photoresponse based on the photothermoelectric (PTE) effect of lead telluride (PbTe) film is demonstrated. Large-area, high-crystallinity PbTe film grown by a low-temperature, CMOS-compatible RF magnetron sputtering method is first reported for photodetection. The PbTe PTE photodetector surpasses the energy band gap limitation, operating even at wavelengths exceeding 10 μm. A rapid response time of less than 1 ms is obtained at 1310 nm, which is superior to those of most other reported PTE detectors. Furthermore, the development of a 5 × 5 array device shows a good photoresponse uniformity and demonstrates consistent mid-infrared imaging capabilities at room temperature. Excellent mechanical flexibility enables the integration of wearable optoelectronic devices. This pioneering research paves the way for significant advancements in Si-based broadband photodetector technologies, with potential applications in monolithic integrated detection and imaging systems that operate in visible- to long-wave infrared wavelengths at room temperature.

ACS PhotonicsVol. 11(11)
University of Electronic Science and Technology of China (CN), Henan Tianguan Group (China) (CN), National Engineering Research Center of Electromagnetic Radiation Control Materials (CN)
National Natural Science Foundation of China, Aeronautical Science Foundation of China, Natural Science Foundation of Sichuan Province
Affordable and clean energy
Openalex Percentile: Top 20%
Advanced Thermoelectric Materials and Devices
1.05
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