Atomically precise copper clusters with dual sites for highly chemoselective and efficient hydroboration
The hydroboration of alkynes into vinylboronate esters is a vital transformation, but achieving high chemoselectivity of targeted functional groups and an appreciable turnover number is a considerable challenge. Herein, we develop two dynamically regulating dual-catalytic-site copper clusters (Cu<sub>4</sub>NC and Cu<sub>8</sub>NC) bearing N-heterocyclic thione ligands that endow Cu<sub>4</sub>NC and Cu<sub>8</sub>NC catalysts with performance. In particular, the performance of microcrystalline Cu<sub>4</sub>NC in hydroboration is characterized by a high turnover number (77786), a high chemoselectivity, high recovery and reusability under mild conditions. Mechanistic studies and density functional theory calculations reveal that, compared with the Cu<sub>8</sub>NC catalyst, the Cu<sub>4</sub>NC catalyst has a lower activation energy for hydroboration, accounting for its high catalytic activity. This work reveals that precisely constructed cluster catalysts with dual catalytic sites may provide a way to substantially improve catalytic properties by fully leveraging synergistic interactions and dynamic ligand effects, thus promoting the development of cluster catalysts.
Authors
- Shuang‐Quan Zang (ORCID: https://orcid.org/0000-0002-6728-0559)
- Chuanxin Sun (ORCID: https://orcid.org/0000-0003-2755-0443)
- Ren‐Wu Huang (ORCID: https://orcid.org/0000-0002-8733-9677)
- Miaomiao Zhang (ORCID: https://orcid.org/0000-0002-4689-1991)
- Xiaoguang Li (ORCID: https://orcid.org/0000-0001-9979-053X)
- Zheng Wang (ORCID: https://orcid.org/0000-0002-7560-2618)
- Yixin Li (ORCID: https://orcid.org/0000-0002-9286-1187)
- Jie Ai
- Teng Jia
- Yue Hua
- Feng Liu
Institutions
- Shenzhen University (CN)
- Henan University of Technology (CN)
- Zhengzhou University (CN)
- Institute for Advanced Study (DE)
- Kunming Institute of Precious Metals (CN)
Publication Details
- Journal
- Nature Communications
- Published
- 2024-11-05
- DOI
- https://doi.org/10.1038/s41467-024-53950-7
- Citations
- 28
- Primary Topic
- Nanocluster Synthesis and Applications
- Type
- article
- Field-Weighted Citation Impact
- 3.28
Funders
- National Natural Science Foundation of China
- National Outstanding Youth Foundation of China