Rapid Chemical Synthesis of High-Entropy Oxide Colloids under Ambient Conditions
High-entropy oxides (HEOs) exhibit high catalytic activities in the O2 evolution reaction (OER). Nevertheless, the methods used for the fabrication of these oxides necessitate the application of heat and/or pressure. Accordingly, herein, HEO colloids are produced by a facile procedure under ambient temperature and pressure conditions using a strong base, an oxidant, and metal salt(s). Using the proposed method, HEO colloids containing up to 12 metal elements are prepared and specifically tailored as electrocatalysts for the OER. This chemical approach enables the cost-effective production of HEO colloids with diverse compositions, opening the door to a wide range of applications of HEOs.
Authors
- Saikat Bolar (ORCID: https://orcid.org/0000-0001-5861-293X)
- Chunyu Yuan (ORCID: https://orcid.org/0009-0009-3906-1816)
- Yoshikazu Ito (ORCID: https://orcid.org/0000-0001-8059-8396)
- Akitaka Ito (ORCID: https://orcid.org/0000-0002-0893-5535)
- Takeshi Fujita (ORCID: https://orcid.org/0000-0002-2318-0433)
Institutions
- University of Tsukuba (JP)
- Kochi University of Technology (JP)
Publication Details
- Journal
- ACS Materials Letters
- Published
- 2024-11-05
- DOI
- https://doi.org/10.1021/acsmaterialslett.4c01849
- Citations
- 3
- Primary Topic
- Catalysis and Oxidation Reactions
- Type
- article
- Field-Weighted Citation Impact
- 0.32
Funders
- Tohoku University
- Japan Society for the Promotion of Science