Rapid Chemical Synthesis of High-Entropy Oxide Colloids under Ambient Conditions

High-entropy oxides (HEOs) exhibit high catalytic activities in the O2 evolution reaction (OER). Nevertheless, the methods used for the fabrication of these oxides necessitate the application of heat and/or pressure. Accordingly, herein, HEO colloids are produced by a facile procedure under ambient temperature and pressure conditions using a strong base, an oxidant, and metal salt(s). Using the proposed method, HEO colloids containing up to 12 metal elements are prepared and specifically tailored as electrocatalysts for the OER. This chemical approach enables the cost-effective production of HEO colloids with diverse compositions, opening the door to a wide range of applications of HEOs.

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Publication Details

Journal
ACS Materials Letters
Published
2024-11-05
DOI
https://doi.org/10.1021/acsmaterialslett.4c01849
Citations
3
Primary Topic
Catalysis and Oxidation Reactions
Type
article
Field-Weighted Citation Impact
0.32

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article

Rapid Chemical Synthesis of High-Entropy Oxide Colloids under Ambient Conditions

Saikat Bolar, Chunyu Yuan, Yoshikazu Ito, Akitaka Ito et al.
3 citations
ACS Materials Letters
Catalysis and Oxidation Reactions
0.32
article

Rapid Chemical Synthesis of High-Entropy Oxide Colloids under Ambient Conditions

Saikat Bolar, Chunyu Yuan, Yoshikazu Ito, Akitaka Ito, Takeshi Fujita
article en
3 citations

Abstract

High-entropy oxides (HEOs) exhibit high catalytic activities in the O2 evolution reaction (OER). Nevertheless, the methods used for the fabrication of these oxides necessitate the application of heat and/or pressure. Accordingly, herein, HEO colloids are produced by a facile procedure under ambient temperature and pressure conditions using a strong base, an oxidant, and metal salt(s). Using the proposed method, HEO colloids containing up to 12 metal elements are prepared and specifically tailored as electrocatalysts for the OER. This chemical approach enables the cost-effective production of HEO colloids with diverse compositions, opening the door to a wide range of applications of HEOs.

ACS Materials LettersVol. 6(12)
University of Tsukuba (JP), Kochi University of Technology (JP)
Tohoku University, Japan Society for the Promotion of Science
Climate action
Openalex Percentile: Top 53%
Catalysis and Oxidation Reactions
0.32
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Rapid Chemical Synthesis of High-Entropy Oxide Colloids under Ambient Conditions — Saikat Bolar, Chunyu Yuan, et al. · ACS Materials Letters (2024) | TGRS Research Map | TGRS