Mid‐Infrared Sensing Using a Hollow–Core Fiber in a Nonlinear Interferometer

Abstract Increasing the interaction path length is a well‐known method for enhancing the sensitivity of the optical detection system. Hollow–core fibers (HCFs) represent a viable alternative to the traditional multi‐path cells offering low optical losses and strong confinement of the optical field. Here, the incorporation of an Antiresonant Hollow–core Fiber (AR‐HCF) section into a nonlinear interferometer, where the AR‐HCF section serves as a gas‐sensing cell operating in the IR range is presented. By exploiting the effect of nonlinear interference, the detection is brought into the more operation‐friendly visible range. The detection of methane (CH 4 ) gas at mid‐IR wavelengths within a half‐meter section of AR‐HCF, with an estimated concentration accuracy of 200 ppm·m is demonstrated. These results represent the combination of two research fields within a single instrument and pave the way for further advancement of quantum‐inspired gas sensing techniques.