Room-temperature modulation of microwave conductivity in ferroelectric-gated correlated oxides

We report the nonvolatile modulation of microwave conductivity in ferroelectric PbZr0.2Ti0.8O3-gated ultrathin LaNiO3/La0.67Sr0.33MnO3 correlated oxide channel visualized by microwave impedance microscopy. Polarization switching is obtained by applying a tip bias above the coercive voltage of the ferroelectric layer. The microwave conductivity of the correlated channel underneath the up- and down-polarized domains has been quantified by finite-element analysis of the tip-sample admittance. At room temperature, a resistance on/off ratio above 100 between the two polarization states is sustained at frequencies up to 1 GHz, which starts to drop at higher frequencies. The frequence-dependence suggests that the conductance modulation originates from ferroelectric field-effect control of carrier density. The modulation is nonvolatile, remaining stable after 6 months of domain writing. Our work is significant for potential applications of oxide-based ferroelectric field-effect transistors in high-frequency nanoelectronics and spintronics.

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Publication Details

Journal
Applied Physics Letters
Published
2024-10-28
DOI
https://doi.org/10.1063/5.0231424
Citations
2
Primary Topic
Ferroelectric and Piezoelectric Materials
Type
article
Field-Weighted Citation Impact
0.23

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article

Room-temperature modulation of microwave conductivity in ferroelectric-gated correlated oxides

Keji Lai, Yifei Hao, Shizai Chu, Shaopeng Feng et al.
2 citations
Applied Physics Letters
Ferroelectric and Piezoelectric Materials
0.23
article

Room-temperature modulation of microwave conductivity in ferroelectric-gated correlated oxides

Keji Lai, Yifei Hao, Shizai Chu, Shaopeng Feng, Xia Hong
article en
2 citations

Abstract

We report the nonvolatile modulation of microwave conductivity in ferroelectric PbZr0.2Ti0.8O3-gated ultrathin LaNiO3/La0.67Sr0.33MnO3 correlated oxide channel visualized by microwave impedance microscopy. Polarization switching is obtained by applying a tip bias above the coercive voltage of the ferroelectric layer. The microwave conductivity of the correlated channel underneath the up- and down-polarized domains has been quantified by finite-element analysis of the tip-sample admittance. At room temperature, a resistance on/off ratio above 100 between the two polarization states is sustained at frequencies up to 1 GHz, which starts to drop at higher frequencies. The frequence-dependence suggests that the conductance modulation originates from ferroelectric field-effect control of carrier density. The modulation is nonvolatile, remaining stable after 6 months of domain writing. Our work is significant for potential applications of oxide-based ferroelectric field-effect transistors in high-frequency nanoelectronics and spintronics.

Applied Physics LettersVol. 125(18)
University of Nebraska–Lincoln (US), The University of Texas at Austin (US)
Welch Foundation, Division of Materials Research
Affordable and clean energy
Openalex Percentile: Top 50%
Ferroelectric and Piezoelectric Materials
0.23
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