Modulating the Electrical Transport in Superconducting NbC Crystals by Fractal Morphology

The self-similar fractal morphology mediated by nonequilibrium processes is widely observed in low-dimensional materials grown by various techniques. Understanding how these fractal geometries affect the physical and chemical properties of materials and devices is crucial for both fundamental studies and various applications. In particular, the interplay between superconducting phase fluctuations and disorder can give rise to intriguing phenomena depending on the dimensionality. However, current experimental studies on low-dimensional superconductors are limited to two- and one-dimensional systems, leaving fractional dimensional systems largely unexplored. Here, we use chemical vapor deposition to successfully synthesize ultrathin NbC crystals with a well-defined fractal geometry at the nanoscale. By performing electrical transport measurements, we find that both the superconducting and normal-state properties are strongly affected in the fractal samples, where the intrinsic and geometric disorder is induced. In contrast to the 2D crystal, the fractal NbC crystals show a significant low-temperature resistive upturn before the onset of superconducting transition, which can be attributed to the disorder-enhanced electron-electron interaction effect. From transport data analysis, we demonstrate that the superconducting transition in NbC is correlated to the strength of disorder and the fractional dimensions, revealing that nanoscale fractal structures can significantly modify the electronic properties of low-dimensional superconductors. Our work paves the way for the explorations of mesoscopic transport and intriguing superconducting phenomena in fractional dimensions.

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Publication Details

Journal
ACS Applied Materials & Interfaces
Published
2024-10-28
DOI
https://doi.org/10.1021/acsami.4c13602
Citations
2
Primary Topic
Surface and Thin Film Phenomena
Type
article
Field-Weighted Citation Impact
0.68

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article

Modulating the Electrical Transport in Superconducting NbC Crystals by Fractal Morphology

Wencai Ren, Su Sun, Chuan Xu, Yunqi Fu et al.
2 citations
ACS Applied Materials & Interfaces
Surface and Thin Film Phenomena
0.68
article

Modulating the Electrical Transport in Superconducting NbC Crystals by Fractal Morphology

Wencai Ren, Su Sun, Chuan Xu, Yunqi Fu, Qiang Wang, Hui–Ming Cheng, Ning Kang, Zhibo Liu, Meng Hao
article en
2 citations

Abstract

The self-similar fractal morphology mediated by nonequilibrium processes is widely observed in low-dimensional materials grown by various techniques. Understanding how these fractal geometries affect the physical and chemical properties of materials and devices is crucial for both fundamental studies and various applications. In particular, the interplay between superconducting phase fluctuations and disorder can give rise to intriguing phenomena depending on the dimensionality. However, current experimental studies on low-dimensional superconductors are limited to two- and one-dimensional systems, leaving fractional dimensional systems largely unexplored. Here, we use chemical vapor deposition to successfully synthesize ultrathin NbC crystals with a well-defined fractal geometry at the nanoscale. By performing electrical transport measurements, we find that both the superconducting and normal-state properties are strongly affected in the fractal samples, where the intrinsic and geometric disorder is induced. In contrast to the 2D crystal, the fractal NbC crystals show a significant low-temperature resistive upturn before the onset of superconducting transition, which can be attributed to the disorder-enhanced electron-electron interaction effect. From transport data analysis, we demonstrate that the superconducting transition in NbC is correlated to the strength of disorder and the fractional dimensions, revealing that nanoscale fractal structures can significantly modify the electronic properties of low-dimensional superconductors. Our work paves the way for the explorations of mesoscopic transport and intriguing superconducting phenomena in fractional dimensions.

ACS Applied Materials & InterfacesVol. 16(44)
University of Science and Technology of China (CN), Chinese Academy of Sciences (CN), Peking University (CN), Hefei University (CN), Shenzhen Institutes of Advanced Technology (CN), Nano Carbon (Poland) (PL)
National Natural Science Foundation of China, Chinese Academy of Sciences, Institute of Metal Research, Chinese Academy of Sciences
Openalex Percentile: Top 30%
Surface and Thin Film Phenomena
0.68
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