Active infrared tuning of metal–insulator-metal resonances by VO2 thin film

VO<sub>2</sub> is a promising phase change material offering a large contrast of electric, thermal, and optical properties when transitioning from semiconductor to metallic phase. Here we show that a hybrid metamaterial obtained by proper combination of a VO<sub>2</sub> layer and a nanodisk gold array provides a tunable plasmonic gap resonance in the infrared range. Specifically, we have designed and fabricated a metal-insulator-metal gap resonance by inserting sub-wavelength VO<sub>2</sub> film between a flat gold layer and a gold nanodisk resonator array. The resonance of the hybrid metamaterial is centered in the useful 3-5 μm range when VO<sub>2</sub> is in its semiconductor state. The experimental study highlights a monotonical spectral tuning of the resonance when increasing temperature up to 50 °C above the room temperature, providing a continuous resonance shift of almost 1 μm in the mid-infrared range. Wavelength range and intensity tunability can be further optimized by modifying the thicknesses of the layers and metamaterial parameters.

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Publication Details

Journal
Scientific Reports
Published
2024-10-25
DOI
https://doi.org/10.1038/s41598-024-75430-0
Citations
7
Primary Topic
Transition Metal Oxide Nanomaterials
Type
article
Field-Weighted Citation Impact
1.18

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article

Active infrared tuning of metal–insulator-metal resonances by VO2 thin film

C. Sibilia, Roberto Macaluso, Emilija Petronijevic, Lucilla Pronti et al.
7 citations
Scientific Reports
Transition Metal Oxide Nanomaterials
1.18
article

Active infrared tuning of metal–insulator-metal resonances by VO2 thin film

C. Sibilia, Roberto Macaluso, Emilija Petronijevic, Lucilla Pronti, Maria Cristina Larciprete, Marco Centini, Roberto Li Voti, Andréa Toma, Luca Razzari, Vincenzo Aglieri
article en
7 citations

Abstract

VO<sub>2</sub> is a promising phase change material offering a large contrast of electric, thermal, and optical properties when transitioning from semiconductor to metallic phase. Here we show that a hybrid metamaterial obtained by proper combination of a VO<sub>2</sub> layer and a nanodisk gold array provides a tunable plasmonic gap resonance in the infrared range. Specifically, we have designed and fabricated a metal-insulator-metal gap resonance by inserting sub-wavelength VO<sub>2</sub> film between a flat gold layer and a gold nanodisk resonator array. The resonance of the hybrid metamaterial is centered in the useful 3-5 μm range when VO<sub>2</sub> is in its semiconductor state. The experimental study highlights a monotonical spectral tuning of the resonance when increasing temperature up to 50 °C above the room temperature, providing a continuous resonance shift of almost 1 μm in the mid-infrared range. Wavelength range and intensity tunability can be further optimized by modifying the thicknesses of the layers and metamaterial parameters.

Scientific ReportsVol. 14(1)
Italian Institute of Technology (IT), Institut National de la Recherche Scientifique (CA), Istituto Nazionale di Fisica Nucleare, Laboratori Nazionali di Frascati (IT), Sapienza University of Rome (IT), University of Palermo (IT)
European Commission
Affordable and clean energy
Openalex Percentile: Top 25%
Transition Metal Oxide Nanomaterials
1.18
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