Low-frequency resistance fluctuations in an ionic-liquid-gated channel probed by cross-correlation noise spectroscopy

A system in equilibrium keeps ``exploring'' nearby states in the phase space and consequently, fluctuations can contain information, that the mean value does not. However, such measurements involve a fairly complex interplay of effects arising in the device and measurement electronics, that are nontrivial to disentangle. In this paper, we briefly analyze some of these issues and show the relevance of a two-amplifier cross-correlation technique for semiconductors and thin films commonly encountered. We show that by using home-built very low-cost amplifiers, one can measure spectral densities as low as approximately ${10}^{\ensuremath{-}18}$--${10}^{\ensuremath{-}19}\phantom{\rule{0.2em}{0ex}}{\mathrm{V}}^{2}\phantom{\rule{0.2em}{0ex}}\mathrm{H}{\mathrm{z}}^{\ensuremath{-}1}$. We apply this method to an ionic-liquid-gated Ga:ZnO channel and show that the glass transition of the ionic liquid brings about a change in the exponent of the low-frequency resistance fluctuations of the conducting channel. The variation is absent in ungated devices. Our analysis suggests that a log-normal distribution of the Debye-relaxation times of the fluctuations and an increased weight of the long-timescale relaxations can give a phenomenological but quantitative explanation of the observed change in the exponent.

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Publication Details

Journal
Physical Review Applied
Published
2024-10-25
DOI
https://doi.org/10.1103/physrevapplied.22.044068
Citations
1
Primary Topic
Electrochemical Analysis and Applications
Type
article
Field-Weighted Citation Impact
0.17
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article

Low-frequency resistance fluctuations in an ionic-liquid-gated channel probed by cross-correlation noise spectroscopy

Buddhadeb Pal, D. A. Ritchie, Bikash C. Barik, Aditya Jain et al.
1 citations
Physical Review Applied
Electrochemical Analysis and Applications
0.17
article

Low-frequency resistance fluctuations in an ionic-liquid-gated channel probed by cross-correlation noise spectroscopy

Buddhadeb Pal, D. A. Ritchie, Bikash C. Barik, Aditya Jain, Himadri Chakraborti, K. Das Gupta, Harvey E. Beere
article en
1 citations

Abstract

A system in equilibrium keeps ``exploring'' nearby states in the phase space and consequently, fluctuations can contain information, that the mean value does not. However, such measurements involve a fairly complex interplay of effects arising in the device and measurement electronics, that are nontrivial to disentangle. In this paper, we briefly analyze some of these issues and show the relevance of a two-amplifier cross-correlation technique for semiconductors and thin films commonly encountered. We show that by using home-built very low-cost amplifiers, one can measure spectral densities as low as approximately ${10}^{\ensuremath{-}18}$--${10}^{\ensuremath{-}19}\phantom{\rule{0.2em}{0ex}}{\mathrm{V}}^{2}\phantom{\rule{0.2em}{0ex}}\mathrm{H}{\mathrm{z}}^{\ensuremath{-}1}$. We apply this method to an ionic-liquid-gated Ga:ZnO channel and show that the glass transition of the ionic liquid brings about a change in the exponent of the low-frequency resistance fluctuations of the conducting channel. The variation is absent in ungated devices. Our analysis suggests that a log-normal distribution of the Debye-relaxation times of the fluctuations and an increased weight of the long-timescale relaxations can give a phenomenological but quantitative explanation of the observed change in the exponent.

Physical Review AppliedVol. 22(4)
Centre National de la Recherche Scientifique (FR), Indian Institute of Technology Bombay (IN), Indian Association for the Cultivation of Science (IN), Royal Holloway University of London (GB), University of Cambridge (GB), Commissariat à l'Énergie Atomique et aux Énergies Alternatives (FR), Université Paris-Saclay (FR), CEA Paris-Saclay (FR)
Affordable and clean energy
Openalex Percentile: Top 58%
Electrochemical Analysis and Applications
0.17
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