Proximity-Induced Superconductivity in a 2D Kondo Lattice of an <i>f</i>-Electron-Based Surface Alloy
Realizing hybrids of low-dimensional Kondo lattices and superconducting substrates leads to fascinating platforms for studying the exciting physics of strongly correlated electron systems with induced superconducting pairing. Here, we report a scanning tunneling microscopy and spectroscopy study of a new type of two-dimensional (2D) La-Ce alloy grown epitaxially on a superconducting Re(0001) substrate. We observe the characteristic spectroscopic signature of a hybridization gap evidencing the coherent spin screening in the 2D Kondo lattice realized by the ultrathin La-Ce alloy film on normal conducting Re(0001). Upon lowering the temperature below the critical temperature of rhenium, a superconducting gap is induced exhibiting an energy asymmetry of the coherence peaks that arises from the interaction of residual unscreened magnetic moments with the superconducting substrate. A positive correlation between the Kondo hybridization gap and the asymmetry of the coherence peaks is found.
Authors
- R. Wiesendanger (ORCID: https://orcid.org/0000-0002-0472-4183)
- Dirk K. Morr (ORCID: https://orcid.org/0000-0003-3692-2835)
- Howon Kim (ORCID: https://orcid.org/0000-0002-3024-129X)
Institutions
- Universität Hamburg (DE)
- University of Illinois Chicago (US)
Publication Details
- Journal
- Nano Letters
- Published
- 2024-10-25
- DOI
- https://doi.org/10.1021/acs.nanolett.4c04796
- Citations
- 1
- Primary Topic
- Rare-earth and actinide compounds
- Type
- article
- Field-Weighted Citation Impact
- 0.31
Funders
- U.S. Department of Energy
- Deutsche Forschungsgemeinschaft
- Office of Science
- Basic Energy Sciences
- H2020 European Research Council