Proximity-Induced Superconductivity in a 2D Kondo Lattice of an <i>f</i>-Electron-Based Surface Alloy

Realizing hybrids of low-dimensional Kondo lattices and superconducting substrates leads to fascinating platforms for studying the exciting physics of strongly correlated electron systems with induced superconducting pairing. Here, we report a scanning tunneling microscopy and spectroscopy study of a new type of two-dimensional (2D) La-Ce alloy grown epitaxially on a superconducting Re(0001) substrate. We observe the characteristic spectroscopic signature of a hybridization gap evidencing the coherent spin screening in the 2D Kondo lattice realized by the ultrathin La-Ce alloy film on normal conducting Re(0001). Upon lowering the temperature below the critical temperature of rhenium, a superconducting gap is induced exhibiting an energy asymmetry of the coherence peaks that arises from the interaction of residual unscreened magnetic moments with the superconducting substrate. A positive correlation between the Kondo hybridization gap and the asymmetry of the coherence peaks is found.

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Publication Details

Journal
Nano Letters
Published
2024-10-25
DOI
https://doi.org/10.1021/acs.nanolett.4c04796
Citations
1
Primary Topic
Rare-earth and actinide compounds
Type
article
Field-Weighted Citation Impact
0.31

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article

Proximity-Induced Superconductivity in a 2D Kondo Lattice of an f-Electron-Based Surface Alloy

R. Wiesendanger, Dirk K. Morr, Howon Kim
1 citations
Nano Letters
Rare-earth and actinide compounds
0.31
article

Proximity-Induced Superconductivity in a 2D Kondo Lattice of an f-Electron-Based Surface Alloy

R. Wiesendanger, Dirk K. Morr, Howon Kim
article en
1 citations

Abstract

Realizing hybrids of low-dimensional Kondo lattices and superconducting substrates leads to fascinating platforms for studying the exciting physics of strongly correlated electron systems with induced superconducting pairing. Here, we report a scanning tunneling microscopy and spectroscopy study of a new type of two-dimensional (2D) La-Ce alloy grown epitaxially on a superconducting Re(0001) substrate. We observe the characteristic spectroscopic signature of a hybridization gap evidencing the coherent spin screening in the 2D Kondo lattice realized by the ultrathin La-Ce alloy film on normal conducting Re(0001). Upon lowering the temperature below the critical temperature of rhenium, a superconducting gap is induced exhibiting an energy asymmetry of the coherence peaks that arises from the interaction of residual unscreened magnetic moments with the superconducting substrate. A positive correlation between the Kondo hybridization gap and the asymmetry of the coherence peaks is found.

Nano LettersVol. 24(44)
Universität Hamburg (DE), University of Illinois Chicago (US)
U.S. Department of Energy, Deutsche Forschungsgemeinschaft, Office of Science, Basic Energy Sciences, H2020 European Research Council
Openalex Percentile: Top 42%
Rare-earth and actinide compounds
0.31
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Proximity-Induced Superconductivity in a 2D Kondo Lattice of an <i>f</i>-Electron-Based Surface Alloy — R. Wiesendanger, Dirk K. Morr, et al. · Nano Letters (2024) | TGRS Research Map | TGRS