Contrasting Domestic and Global Impacts of Emission Reductions in China on Tropospheric Ozone

Abstract Sustained near‐surface ozone pollution despite stringent emission controls in China has drawn wide attention. However, how such rapid regional emission reductions affect global tropospheric ozone remains unexplored. Here, using an ensemble of measurements and global model simulations, we find Chinese emission reductions during 2013–2020 have increased domestic surface ozone; particularly in North China, they have decreased the global tropospheric ozone burden by 2.7 Tg (54% of China's anthropogenic contribution and 7% of global anthropogenic contribution in 2019) and ozone radiative forcing by 8.8 mW m −2 (64% of China's anthropogenic contribution and 9% of global anthropogenic contribution in 2019). Nitrogen oxides (NO x ) associated nonlinear chemistry and height‐dependent atmospheric transport patterns primarily cause the contrasting impacts. Future Chinese NO x emission controls would continue to decrease global tropospheric ozone, while regional surface ozone may still increase unless NO x reductions exceed ∼53% of the 2019 level. Our results reveal the substantial benefit of regional emission reductions in China on global tropospheric ozone mitigation.

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Publication Details

Journal
Journal of Geophysical Research Atmospheres
Published
2024-10-25
DOI
https://doi.org/10.1029/2024jd041453
Citations
6
Primary Topic
Atmospheric chemistry and aerosols
Type
article
Field-Weighted Citation Impact
2.26

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article

Contrasting Domestic and Global Impacts of Emission Reductions in China on Tropospheric Ozone

Xiao Lu, Xiaolin Wang, Han Han, Lin Zhang
6 citations
Journal of Geophysical Research Atmospheres
Atmospheric chemistry and aerosols
2.26
article

Contrasting Domestic and Global Impacts of Emission Reductions in China on Tropospheric Ozone

Xiao Lu, Xiaolin Wang, Han Han, Lin Zhang
article en
6 citations

Abstract

Abstract Sustained near‐surface ozone pollution despite stringent emission controls in China has drawn wide attention. However, how such rapid regional emission reductions affect global tropospheric ozone remains unexplored. Here, using an ensemble of measurements and global model simulations, we find Chinese emission reductions during 2013–2020 have increased domestic surface ozone; particularly in North China, they have decreased the global tropospheric ozone burden by 2.7 Tg (54% of China's anthropogenic contribution and 7% of global anthropogenic contribution in 2019) and ozone radiative forcing by 8.8 mW m −2 (64% of China's anthropogenic contribution and 9% of global anthropogenic contribution in 2019). Nitrogen oxides (NO x ) associated nonlinear chemistry and height‐dependent atmospheric transport patterns primarily cause the contrasting impacts. Future Chinese NO x emission controls would continue to decrease global tropospheric ozone, while regional surface ozone may still increase unless NO x reductions exceed ∼53% of the 2019 level. Our results reveal the substantial benefit of regional emission reductions in China on global tropospheric ozone mitigation.

Journal of Geophysical Research AtmospheresVol. 129(20)
Harvard University (US), Sun Yat-sen University (CN), Peking University (CN), Southern Marine Science and Engineering Guangdong Laboratory (Guangzhou) (CN)
China Postdoctoral Science Foundation, Peking University, National Key Research and Development Program of China
Openalex Percentile: Top 12%
Atmospheric chemistry and aerosols
2.26
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