Van der Waals exciton polaritons with linewidth approaching homogeneous limit

Van der Waals semiconductors have provided a new platform to extend the physics and applications of cavity exciton polaritons, thanks to their flexibility of integration, large oscillator strength, and novel moir\'e physics. However, the inhomogeneous broadening of excitons, originating from strain, defect, or interface fluctuation, has been an obstacle to further exploring coherent quantum phenomena and devices in this community. In this work, we show that the contribution of exciton inhomogeneous broadening to polariton linewidth can be fully suppressed by increasing Rabi splitting. The results can be well reproduced theoretically- by modeling the excitonphoton coupling using a non-Hermitian Hamiltonian. Our findings not only shed light on the development of coherent Van der Waals polariton devices but also demonstrate a general conclusion on the correlation between the inhomogeneous broadening of a solid-state oscillator and the linewidth of its corresponding light-matter hybrids.

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Publication Details

Journal
Physical Review Materials
Published
2024-10-24
DOI
https://doi.org/10.1103/physrevmaterials.8.l101002
Citations
2
Primary Topic
Strong Light-Matter Interactions
Type
article
Field-Weighted Citation Impact
0.68

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article

Van der Waals exciton polaritons with linewidth approaching homogeneous limit

Yuquan Zhou, Hongming Zhang, Hang Zhou, Haochen Wang et al.
2 citations
Physical Review Materials
Strong Light-Matter Interactions
0.68
article

Van der Waals exciton polaritons with linewidth approaching homogeneous limit

Yuquan Zhou, Hongming Zhang, Hang Zhou, Haochen Wang, Zhanghai Chen, Xin Li, Long Zhang, Song Luo, Yaofeng Zhu
article en
2 citations

Abstract

Van der Waals semiconductors have provided a new platform to extend the physics and applications of cavity exciton polaritons, thanks to their flexibility of integration, large oscillator strength, and novel moir\'e physics. However, the inhomogeneous broadening of excitons, originating from strain, defect, or interface fluctuation, has been an obstacle to further exploring coherent quantum phenomena and devices in this community. In this work, we show that the contribution of exciton inhomogeneous broadening to polariton linewidth can be fully suppressed by increasing Rabi splitting. The results can be well reproduced theoretically- by modeling the excitonphoton coupling using a non-Hermitian Hamiltonian. Our findings not only shed light on the development of coherent Van der Waals polariton devices but also demonstrate a general conclusion on the correlation between the inhomogeneous broadening of a solid-state oscillator and the linewidth of its corresponding light-matter hybrids.

Physical Review MaterialsVol. 8(10)
Xiamen University (CN), Xiamen University of Technology (CN)
National Natural Science Foundation of China, National Key Research and Development Program of China
Climate action
Openalex Percentile: Top 30%
Strong Light-Matter Interactions
0.68
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Van der Waals exciton polaritons with linewidth approaching homogeneous limit — Yuquan Zhou, Hongming Zhang, et al. · Physical Review Materials (2024) | TGRS Research Map | TGRS