Characterizing the diffuse continuum excitations in the classical spin liquid <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:mi>h</mml:mi><mml:mtext>−</mml:mtext><mml:msub><mml:mi>YMnO</mml:mi><mml:mn>3</mml:mn></mml:msub></m

We extend previous inelastic neutron scattering results on the geometrically frustrated antiferromagnet hexagonal-<a:math xmlns:a="http://www.w3.org/1998/Math/MathML"><a:msub><a:mi>YMnO</a:mi><a:mn>3</a:mn></a:msub></a:math>, which has been suggested to belong to the class of classical spin liquids. We expand the energy transfer range of the diffuse signal up to 6.9 meV within a wide temperature range around the ordering temperature, <b:math xmlns:b="http://www.w3.org/1998/Math/MathML"><b:msub><b:mi>T</b:mi><b:mi mathvariant="normal">N</b:mi></b:msub></b:math>. The two distinct diffuse signals in the <d:math xmlns:d="http://www.w3.org/1998/Math/MathML"><d:mrow><d:mi>a</d:mi><d:mtext>−</d:mtext><d:mi>b</d:mi></d:mrow></d:math> plane, the signal localized at <e:math xmlns:e="http://www.w3.org/1998/Math/MathML"><e:msup><e:mi mathvariant="normal">Γ</e:mi><e:mo>′</e:mo></e:msup></e:math> and the scattering intensity connecting <g:math xmlns:g="http://www.w3.org/1998/Math/MathML"><g:msup><g:mi mathvariant="normal">Γ</g:mi><g:mo>′</g:mo></g:msup></g:math> points over the <i:math xmlns:i="http://www.w3.org/1998/Math/MathML"><i:msup><i:mi mathvariant="normal">M</i:mi><i:mo>′</i:mo></i:msup></i:math>, are shown to be only weakly energy dependent. In addition, an external magnetic field of up to 10.5 T applied along <k:math xmlns:k="http://www.w3.org/1998/Math/MathML"><k:mi>c</k:mi></k:math> is shown to have no effect on the diffuse signal. In the orthogonal scattering plane, the signals are shown to be dependent on <l:math xmlns:l="http://www.w3.org/1998/Math/MathML"><l:mi>l</l:mi></l:math> only through the magnetic form factor, showing that the correlations are purely two-dimensional, and supporting the origin of this to be the frustrated <m:math xmlns:m="http://www.w3.org/1998/Math/MathML"><m:msup><m:mrow><m:mi>Mn</m:mi></m:mrow><m:mrow><m:mn>3</m:mn><m:mo>+</m:mo></m:mrow></m:msup></m:math> triangles. This result is corroborated by atomistic spin dynamics simulations showing similar scattering vector and temperature behaviors. Lastly, data for the spin wave scattering in the <n:math xmlns:n="http://www.w3.org/1998/Math/MathML"><n:mrow><n:mo>(</n:mo><n:mi>h</n:mi><n:mo>,</n:mo><n:mn>0</n:mn><n:mo>,</n:mo><n:mi>l</n:mi><n:mo>)</n:mo></n:mrow></n:math> plane allow for a discussion of the magnetic ground state where better agreement is found between the data and an ordered structure of the <o:math xmlns:o="http://www.w3.org/1998/Math/MathML"><o:msub><o:mi mathvariant="normal">Γ</o:mi><o:mn>1</o:mn></o:msub></o:math> or <q:math xmlns:q="http://www.w3.org/1998/Math/MathML"><q:msub><q:mi mathvariant="normal">Γ</q:mi><q:mn>3</q:mn></q:msub></q:math> symmetry, albeit crystal electric field arguments dismiss the <s:math xmlns:s="http://www.w3.org/1998/Math/MathML"><s:msub><s:mi mathvariant="normal">Γ</s:mi><s:mn>1</s:mn></s:msub></s:math> as a possibility. Published by the American Physical Society 2024

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Journal
Physical review. B./Physical review. B
Published
2024-10-18
DOI
https://doi.org/10.1103/physrevb.110.144429
Citations
2
Primary Topic
Advanced Condensed Matter Physics
Type
article
Field-Weighted Citation Impact
0.62

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article

Characterizing the diffuse continuum excitations in the classical spin liquid <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:mi>h</mml:mi><mml:mtext>−</mml:mtext><mml:msub><mml:mi>YMnO</mml:mi><mml:mn>3</mml:mn></mml:msub></m

D. Prabhakaran, Tara N. Tošić, Jakob Lass, Sofie Holm-Janas et al.
2 citations
Physical review. B./Physical review. B
Advanced Condensed Matter Physics
0.62
article

Characterizing the diffuse continuum excitations in the classical spin liquid <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:mi>h</mml:mi><mml:mtext>−</mml:mtext><mml:msub><mml:mi>YMnO</mml:mi><mml:mn>3</mml:mn></mml:msub></m

D. Prabhakaran, Tara N. Tošić, Jakob Lass, Sofie Holm-Janas, Kristine M. L. Krighaar, P. P. Deen, Kim Lefmann, Emma Y. Lenander
article en
2 citations

Abstract

We extend previous inelastic neutron scattering results on the geometrically frustrated antiferromagnet hexagonal-<a:math xmlns:a="http://www.w3.org/1998/Math/MathML"><a:msub><a:mi>YMnO</a:mi><a:mn>3</a:mn></a:msub></a:math>, which has been suggested to belong to the class of classical spin liquids. We expand the energy transfer range of the diffuse signal up to 6.9 meV within a wide temperature range around the ordering temperature, <b:math xmlns:b="http://www.w3.org/1998/Math/MathML"><b:msub><b:mi>T</b:mi><b:mi mathvariant="normal">N</b:mi></b:msub></b:math>. The two distinct diffuse signals in the <d:math xmlns:d="http://www.w3.org/1998/Math/MathML"><d:mrow><d:mi>a</d:mi><d:mtext>−</d:mtext><d:mi>b</d:mi></d:mrow></d:math> plane, the signal localized at <e:math xmlns:e="http://www.w3.org/1998/Math/MathML"><e:msup><e:mi mathvariant="normal">Γ</e:mi><e:mo>′</e:mo></e:msup></e:math> and the scattering intensity connecting <g:math xmlns:g="http://www.w3.org/1998/Math/MathML"><g:msup><g:mi mathvariant="normal">Γ</g:mi><g:mo>′</g:mo></g:msup></g:math> points over the <i:math xmlns:i="http://www.w3.org/1998/Math/MathML"><i:msup><i:mi mathvariant="normal">M</i:mi><i:mo>′</i:mo></i:msup></i:math>, are shown to be only weakly energy dependent. In addition, an external magnetic field of up to 10.5 T applied along <k:math xmlns:k="http://www.w3.org/1998/Math/MathML"><k:mi>c</k:mi></k:math> is shown to have no effect on the diffuse signal. In the orthogonal scattering plane, the signals are shown to be dependent on <l:math xmlns:l="http://www.w3.org/1998/Math/MathML"><l:mi>l</l:mi></l:math> only through the magnetic form factor, showing that the correlations are purely two-dimensional, and supporting the origin of this to be the frustrated <m:math xmlns:m="http://www.w3.org/1998/Math/MathML"><m:msup><m:mrow><m:mi>Mn</m:mi></m:mrow><m:mrow><m:mn>3</m:mn><m:mo>+</m:mo></m:mrow></m:msup></m:math> triangles. This result is corroborated by atomistic spin dynamics simulations showing similar scattering vector and temperature behaviors. Lastly, data for the spin wave scattering in the <n:math xmlns:n="http://www.w3.org/1998/Math/MathML"><n:mrow><n:mo>(</n:mo><n:mi>h</n:mi><n:mo>,</n:mo><n:mn>0</n:mn><n:mo>,</n:mo><n:mi>l</n:mi><n:mo>)</n:mo></n:mrow></n:math> plane allow for a discussion of the magnetic ground state where better agreement is found between the data and an ordered structure of the <o:math xmlns:o="http://www.w3.org/1998/Math/MathML"><o:msub><o:mi mathvariant="normal">Γ</o:mi><o:mn>1</o:mn></o:msub></o:math> or <q:math xmlns:q="http://www.w3.org/1998/Math/MathML"><q:msub><q:mi mathvariant="normal">Γ</q:mi><q:mn>3</q:mn></q:msub></q:math> symmetry, albeit crystal electric field arguments dismiss the <s:math xmlns:s="http://www.w3.org/1998/Math/MathML"><s:msub><s:mi mathvariant="normal">Γ</s:mi><s:mn>1</s:mn></s:msub></s:math> as a possibility. Published by the American Physical Society 2024

Physical review. B./Physical review. BVol. 110(14)
University of Copenhagen (DK), European Spallation Source (SE), ETH Zurich (CH), University of Oxford (GB), École Polytechnique Fédérale de Lausanne (CH), Technical University of Denmark (DK)
European Commission, Eidgenössische Technische Hochschule Zürich, Paul Scherrer Institut, DanScatt, Engineering and Physical Sciences Research Council, National Supercomputing Center, Korea Institute of Science and Technology Information, H2020 European Research Council
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Openalex Percentile: Top 32%
Advanced Condensed Matter Physics
0.62
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