Temperature dependence of irradiation-induced amorphization in a high-entropy titanate pyrochlore

Abstract The temperature dependence of amorphization in a high-entropy pyrochlore, (Yb 0.2 Tm 0.2 Lu 0.2 Ho 0.2 Er 0.2 ) 2 Ti 2 O 7 , under irradiation with 600 keV Xe ions has been studied using in situ transmission electron microscopy (TEM). The critical amorphization dose increases with temperature, and the critical temperature for amorphization is 800 K. At room temperature, the critical amorphization dose is larger than that previously determined for this pyrochlore under bulk-like 4 MeV Au ion irradiation but is similar to the critical doses determined in two other high-entropy titanate pyrochlores under 800 keV Kr ion irradiation using in situ TEM, which is consistent with reported behavior in simple rare-earth titanate pyrochlores. Graphical abstract

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Publication Details

Journal
MRS Communications
Published
2024-10-18
DOI
https://doi.org/10.1557/s43579-024-00648-y
Citations
6
Primary Topic
Nuclear materials and radiation effects
Type
article
Field-Weighted Citation Impact
0.70

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article

Temperature dependence of irradiation-induced amorphization in a high-entropy titanate pyrochlore

Veerle Keppens, Anamul H. Mir, William J. Weber, Candice Kinsler-Fedon et al.
6 citations
MRS Communications
Nuclear materials and radiation effects
0.70
article

Temperature dependence of irradiation-induced amorphization in a high-entropy titanate pyrochlore

Veerle Keppens, Anamul H. Mir, William J. Weber, Candice Kinsler-Fedon, Yanwen Zhang
article en
6 citations

Abstract

Abstract The temperature dependence of amorphization in a high-entropy pyrochlore, (Yb 0.2 Tm 0.2 Lu 0.2 Ho 0.2 Er 0.2 ) 2 Ti 2 O 7 , under irradiation with 600 keV Xe ions has been studied using in situ transmission electron microscopy (TEM). The critical amorphization dose increases with temperature, and the critical temperature for amorphization is 800 K. At room temperature, the critical amorphization dose is larger than that previously determined for this pyrochlore under bulk-like 4 MeV Au ion irradiation but is similar to the critical doses determined in two other high-entropy titanate pyrochlores under 800 keV Kr ion irradiation using in situ TEM, which is consistent with reported behavior in simple rare-earth titanate pyrochlores. Graphical abstract

MRS CommunicationsVol. 14(6)
University of Huddersfield (GB), Queen's University (CA), University of Tennessee at Knoxville (US)
National Science Foundation, Government of Canada, Canada Excellence Research Chairs, Government of Canada, UK National Ion Beam Centre, Engineering and Physical Sciences Research Council, Division of Materials Research
Openalex Percentile: Top 29%
Nuclear materials and radiation effects
0.70
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Temperature dependence of irradiation-induced amorphization in a high-entropy titanate pyrochlore — Veerle Keppens, Anamul H. Mir, et al. · MRS Communications (2024) | TGRS Research Map | TGRS