Origin of Reliable High-Power Performances of PbZr<sub>0.5</sub>Ti<sub>0.5</sub>O<sub>3</sub>–Pb(Mn<sub>1/3</sub>Nb<sub>2/3</sub>)O<sub>3</sub>-Based Piezoelectric Ceramics
High-power piezoelectric ceramics typically operate under severe conditions. This makes the accurate evaluation of their high-power performances through pure quasi-static parameters challenging. The 0.94PbZr<sub>0.5</sub>Ti<sub>0.5</sub>O<sub>3</sub> - 0.06Pb(Mn<sub>1/3</sub>Nb<sub>2/3</sub>)O<sub>3</sub> + 0.005Fe<sub>2</sub>O<sub>3</sub> + 0.002Sc<sub>2</sub>O<sub>3</sub> (PZT-1) ceramic exhibits exceptional and reliable high-power performances at elevated temperatures and under loading conditions. While numerous PZT-based ceramics demonstrate excellent quasi-static parameters, only the PZT-1 ceramic displays superior high-field parameters, such as a low tan δ of 0.97% at 566 V/mm (1 kHz) and a large <i>Q</i><sub>m</sub> of 1164 at 50 V/mm (100 kHz). Therefore, the PZT-1 ceramic demonstrates remarkably slow heat generation and the highest surface temperatures are only 41.8 °C at 50 V/mm (100 kHz). Moreover, the PZT-1 ceramic shows a minimal resonance frequency variation of -0.04% in the temperature range of 25-120 °C at 50 V/mm. Consequently, the PZT-1 ceramic maintains a high and reliable vibration velocity of 0.90 m/s at 120 °C for 30 min, and the ceramic cantilever sustains a high amplitude of 7 μm, significantly outperforming other ceramics. This study conclusively demonstrates that high-field parameters, rather than quasi-static parameters, are more effective in accurately estimating the high-power performances of ceramics.
Authors
- Guoliang Yuan (ORCID: https://orcid.org/0000-0002-1367-267X)
- Shan‐Tao Zhang (ORCID: https://orcid.org/0000-0002-6291-0363)
- Hongdi Wu (ORCID: https://orcid.org/0009-0009-0421-080X)
- Ying Yang (ORCID: https://orcid.org/0000-0002-4810-2976)
- Guanglei Xiang
- Yuequn Wang (ORCID: https://orcid.org/0000-0001-6036-0188)
- Yiping Wang (ORCID: https://orcid.org/0000-0003-4777-9093)
- Zhiyong Pan
- Wenbin Tang
- Xuefeng Zhao (ORCID: https://orcid.org/0000-0001-7262-4064)
- Yaojin Wang (ORCID: https://orcid.org/0000-0003-2561-1855)
- Zhiqin Zeng
Institutions
- Nanjing University of Science and Technology (CN)
- Hangzhou Institute of Applied Acoustics (CN)
- Nanjing University (CN)
- Nanjing University of Aeronautics and Astronautics (CN)
Publication Details
- Journal
- ACS Applied Materials & Interfaces
- Published
- 2024-10-17
- DOI
- https://doi.org/10.1021/acsami.4c12838
- Citations
- 7
- Primary Topic
- Ferroelectric and Piezoelectric Materials
- Type
- article
- Field-Weighted Citation Impact
- 0.82
Funders
- National Natural Science Foundation of China
- Fundamental Research Funds for the Central Universities