Origin of Reliable High-Power Performances of PbZr<sub>0.5</sub>Ti<sub>0.5</sub>O<sub>3</sub>–Pb(Mn<sub>1/3</sub>Nb<sub>2/3</sub>)O<sub>3</sub>-Based Piezoelectric Ceramics

High-power piezoelectric ceramics typically operate under severe conditions. This makes the accurate evaluation of their high-power performances through pure quasi-static parameters challenging. The 0.94PbZr<sub>0.5</sub>Ti<sub>0.5</sub>O<sub>3</sub> - 0.06Pb(Mn<sub>1/3</sub>Nb<sub>2/3</sub>)O<sub>3</sub> + 0.005Fe<sub>2</sub>O<sub>3</sub> + 0.002Sc<sub>2</sub>O<sub>3</sub> (PZT-1) ceramic exhibits exceptional and reliable high-power performances at elevated temperatures and under loading conditions. While numerous PZT-based ceramics demonstrate excellent quasi-static parameters, only the PZT-1 ceramic displays superior high-field parameters, such as a low tan δ of 0.97% at 566 V/mm (1 kHz) and a large <i>Q</i><sub>m</sub> of 1164 at 50 V/mm (100 kHz). Therefore, the PZT-1 ceramic demonstrates remarkably slow heat generation and the highest surface temperatures are only 41.8 °C at 50 V/mm (100 kHz). Moreover, the PZT-1 ceramic shows a minimal resonance frequency variation of -0.04% in the temperature range of 25-120 °C at 50 V/mm. Consequently, the PZT-1 ceramic maintains a high and reliable vibration velocity of 0.90 m/s at 120 °C for 30 min, and the ceramic cantilever sustains a high amplitude of 7 μm, significantly outperforming other ceramics. This study conclusively demonstrates that high-field parameters, rather than quasi-static parameters, are more effective in accurately estimating the high-power performances of ceramics.

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Publication Details

Journal
ACS Applied Materials & Interfaces
Published
2024-10-17
DOI
https://doi.org/10.1021/acsami.4c12838
Citations
7
Primary Topic
Ferroelectric and Piezoelectric Materials
Type
article
Field-Weighted Citation Impact
0.82

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article

Origin of Reliable High-Power Performances of PbZr0.5Ti0.5O3–Pb(Mn1/3Nb2/3)O3-Based Piezoelectric Ceramics

Guoliang Yuan, Shan‐Tao Zhang, Hongdi Wu, Ying Yang, Guanglei Xiang, Yuequn Wang, Yiping Wang, Zhiyong Pan, Wenbin Tang, Xuefeng Zhao, Yaojin Wang, Zhiqin Zeng
article en
7 citations

Abstract

High-power piezoelectric ceramics typically operate under severe conditions. This makes the accurate evaluation of their high-power performances through pure quasi-static parameters challenging. The 0.94PbZr<sub>0.5</sub>Ti<sub>0.5</sub>O<sub>3</sub> - 0.06Pb(Mn<sub>1/3</sub>Nb<sub>2/3</sub>)O<sub>3</sub> + 0.005Fe<sub>2</sub>O<sub>3</sub> + 0.002Sc<sub>2</sub>O<sub>3</sub> (PZT-1) ceramic exhibits exceptional and reliable high-power performances at elevated temperatures and under loading conditions. While numerous PZT-based ceramics demonstrate excellent quasi-static parameters, only the PZT-1 ceramic displays superior high-field parameters, such as a low tan δ of 0.97% at 566 V/mm (1 kHz) and a large <i>Q</i><sub>m</sub> of 1164 at 50 V/mm (100 kHz). Therefore, the PZT-1 ceramic demonstrates remarkably slow heat generation and the highest surface temperatures are only 41.8 °C at 50 V/mm (100 kHz). Moreover, the PZT-1 ceramic shows a minimal resonance frequency variation of -0.04% in the temperature range of 25-120 °C at 50 V/mm. Consequently, the PZT-1 ceramic maintains a high and reliable vibration velocity of 0.90 m/s at 120 °C for 30 min, and the ceramic cantilever sustains a high amplitude of 7 μm, significantly outperforming other ceramics. This study conclusively demonstrates that high-field parameters, rather than quasi-static parameters, are more effective in accurately estimating the high-power performances of ceramics.

ACS Applied Materials & InterfacesVol. 16(43)
Nanjing University of Science and Technology (CN), Hangzhou Institute of Applied Acoustics (CN), Nanjing University (CN), Nanjing University of Aeronautics and Astronautics (CN)
National Natural Science Foundation of China, Fundamental Research Funds for the Central Universities
Openalex Percentile: Top 26%
Ferroelectric and Piezoelectric Materials
0.82
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