Sedimentological Characteristics of <sup>239+240</sup>Pu and <sup>137</sup>Cs in the Sedimentary Deposits of Poyang Lake

The spatial and vertical distribution of 239+240Pu and 137Cs in sediments of Poyang Lake was studied to assess the dynamics of disposition and the pollution status. The activities of 239+240Pu and 137Cs in surface sediments ranged from 0.005 to 0.616 Bq/kg and from 0.70 to 5.82 Bq/kg, respectively. The inventories of 239+240Pu in sediment cores of PYA and PYB were determined to be 75.2 and 19.9 Bq/m2, respectively. In sediment core PYA, the activity of 239+240Pu ranged from 0.043 to 0.485 Bq/kg, while that for 137Cs ranged from 0.39 to 6.80 Bq/kg. An accumulation peak along with two secondary peaks was observed in sediment core PYA, suggesting a correlation between the timing of these subpeaks and flood events in Poyang Lake. By employing 239+240Pu, the average deposition rate for core PYA was calculated as 0.79 cm/year from 1954 to 1998 and as 0.44 cm/year from 1998 to 2022. The results also suggested that the deposition rate of Poyang Lake has been impacted by human activities, such as the construction of water conservancy projects around Poyang Lake and the commissioning of the Three Gorges Dam Project.

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Journal
ACS Earth and Space Chemistry
Published
2024-10-11
DOI
https://doi.org/10.1021/acsearthspacechem.4c00169
Primary Topic
Radioactive contamination and transfer
Type
article
Field-Weighted Citation Impact
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article

Sedimentological Characteristics of 239+240Pu and 137Cs in the Sedimentary Deposits of Poyang Lake

Liangjia Cui, Xiaomin Wei, Zichen Guo, Yongjing Guan et al.
ACS Earth and Space Chemistry
Radioactive contamination and transfer
article

Sedimentological Characteristics of 239+240Pu and 137Cs in the Sedimentary Deposits of Poyang Lake

Liangjia Cui, Xiaomin Wei, Zichen Guo, Yongjing Guan, Kaidi Fan, Haoxuan Chen, Yiyu Lu, Huijuan Wang, Chunping Huang, Xingyu Liu
article en

Abstract

The spatial and vertical distribution of 239+240Pu and 137Cs in sediments of Poyang Lake was studied to assess the dynamics of disposition and the pollution status. The activities of 239+240Pu and 137Cs in surface sediments ranged from 0.005 to 0.616 Bq/kg and from 0.70 to 5.82 Bq/kg, respectively. The inventories of 239+240Pu in sediment cores of PYA and PYB were determined to be 75.2 and 19.9 Bq/m2, respectively. In sediment core PYA, the activity of 239+240Pu ranged from 0.043 to 0.485 Bq/kg, while that for 137Cs ranged from 0.39 to 6.80 Bq/kg. An accumulation peak along with two secondary peaks was observed in sediment core PYA, suggesting a correlation between the timing of these subpeaks and flood events in Poyang Lake. By employing 239+240Pu, the average deposition rate for core PYA was calculated as 0.79 cm/year from 1954 to 1998 and as 0.44 cm/year from 1998 to 2022. The results also suggested that the deposition rate of Poyang Lake has been impacted by human activities, such as the construction of water conservancy projects around Poyang Lake and the commissioning of the Three Gorges Dam Project.

ACS Earth and Space ChemistryVol. 8(11)
Guangxi University (CN)
National Natural Science Foundation of China, National College Students Innovation and Entrepreneurship Training Program
Openalex Percentile: Top 84%
Radioactive contamination and transfer
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