Low-Temperature Production of Battery Grade Graphite from Coal with Recovery and Reuse of the Catalyst
Synthetic graphite is made predominantly from a petroleum-derived needle coke using the Acheson method. This involves heating the needle coke at elevated temperatures of ~ 3000 °C for more than 7 days. High-temperature heating is the most technically challenging, expensive, and energy-intensive aspect of graphite manufacturing. We will present a strategy for synthesizing high-quality battery-grade graphite powder from coal using a low-temperature catalytic graphitization process. The use of a catalyst drops the processing temperatures to 1500 °C and processing times to a few hours. The graphite produced with this process has been tested as a battery anode and has been shown to outperform anodes made with commercially sourced graphite materials. We will also present a sustainable method to recover and reuse the catalyst and acid used to retrieve the catalyst. This overcomes a long-standing technical hurdle associated with using catalysts for manufacturing graphite.
Authors
- YunYang Lee
- Christopher Matranga (ORCID: https://orcid.org/0000-0001-7082-5938)
- Congjun Wang (ORCID: https://orcid.org/0000-0002-3831-2929)
- Yuan Gao (ORCID: https://orcid.org/0000-0001-5198-7640)
- Ki‐Joong Kim (ORCID: https://orcid.org/0000-0001-9374-8103)
- Viet Hung Pham (ORCID: https://orcid.org/0000-0002-2189-7828)
- Ngoc Huynh
Institutions
- National Energy Technology Laboratory (US)
Publication Details
- Published
- 2024-10-09
- DOI
- https://doi.org/10.2172/2460429
- Primary Topic
- Extraction and Separation Processes
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- U.S. Department of Energy
- National Energy Technology Laboratory