Low-Temperature Production of Battery Grade Graphite from Coal with Recovery and Reuse of the Catalyst

Synthetic graphite is made predominantly from a petroleum-derived needle coke using the Acheson method. This involves heating the needle coke at elevated temperatures of ~ 3000 °C for more than 7 days. High-temperature heating is the most technically challenging, expensive, and energy-intensive aspect of graphite manufacturing. We will present a strategy for synthesizing high-quality battery-grade graphite powder from coal using a low-temperature catalytic graphitization process. The use of a catalyst drops the processing temperatures to 1500 °C and processing times to a few hours. The graphite produced with this process has been tested as a battery anode and has been shown to outperform anodes made with commercially sourced graphite materials. We will also present a sustainable method to recover and reuse the catalyst and acid used to retrieve the catalyst. This overcomes a long-standing technical hurdle associated with using catalysts for manufacturing graphite.

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Published
2024-10-09
DOI
https://doi.org/10.2172/2460429
Primary Topic
Extraction and Separation Processes
Type
article
Field-Weighted Citation Impact
0.00

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article

Low-Temperature Production of Battery Grade Graphite from Coal with Recovery and Reuse of the Catalyst

YunYang Lee, Christopher Matranga, Congjun Wang, Yuan Gao et al.
Extraction and Separation Processes
article

Low-Temperature Production of Battery Grade Graphite from Coal with Recovery and Reuse of the Catalyst

YunYang Lee, Christopher Matranga, Congjun Wang, Yuan Gao, Ki‐Joong Kim, Viet Hung Pham, Ngoc Huynh
article en

Abstract

Synthetic graphite is made predominantly from a petroleum-derived needle coke using the Acheson method. This involves heating the needle coke at elevated temperatures of ~ 3000 °C for more than 7 days. High-temperature heating is the most technically challenging, expensive, and energy-intensive aspect of graphite manufacturing. We will present a strategy for synthesizing high-quality battery-grade graphite powder from coal using a low-temperature catalytic graphitization process. The use of a catalyst drops the processing temperatures to 1500 °C and processing times to a few hours. The graphite produced with this process has been tested as a battery anode and has been shown to outperform anodes made with commercially sourced graphite materials. We will also present a sustainable method to recover and reuse the catalyst and acid used to retrieve the catalyst. This overcomes a long-standing technical hurdle associated with using catalysts for manufacturing graphite.

National Energy Technology Laboratory (US)
U.S. Department of Energy, National Energy Technology Laboratory
Openalex Percentile: Top 83%
Extraction and Separation Processes
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Low-Temperature Production of Battery Grade Graphite from Coal with Recovery and Reuse of the Catalyst — YunYang Lee, Christopher Matranga, et al. · (2024) | TGRS Research Map | TGRS